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IASI observations of sulfur dioxide (SO2) in the boundary layer of Norilsk
Open accessAbstract
Norilsk is one of the most polluted cities in the world, largely because of intense mining of heavy metals. Here we present satellite observations of SO 2 in a large area surrounding the city, derived from 4 years of measurements from the Infrared Atmospheric Sounding Interferometer (IASI), the nadir thermal infrared (TIR) sounder onboard the MetOp platforms. TIR instruments are conventionally considered to be inadequate for monitoring near‐surface composition, because their sensitivity to the lowest part of the atmosphere is limited by the thermal contrast between the ground and the air above it. We demonstrate that IASI is capable of measuring SO 2 (here as a partial column from 0 to 2 km) in Norilsk, thanks to the large temperature inversions and the low humidity in wintertime. We discuss the influence of thermal contrast and of surface humidity on the SO 2 retrieved columns and estimate the retrieval errors. Using a simple box model, we derive the yearly total emissions of SO 2 from Norilsk and compare them to previously reported values. More generally, we present in this work the first large‐scale demonstration of the capability of space‐based TIR sounders to measure near‐surface SO 2 anthropogenic pollution.
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Since the onset of Eurasia's heavy industrialisation in the 1930s, pollution from the Norilsk mining complex has destroyed vast areas of pristine taiga and tundra habitats on the Taimyr Peninsula.
“Since the onset of Eurasia's heavy industrialisation in the 1930s, pollution from the Norilsk mining complex (Kharuk et al. 1996) has destroyed vast areas of pristine taiga and tundra habitats on the Taimyr Peninsula (Bauduin et al ., 2014; Korets et al ., 2014).”
From Ecological and conceptual consequences of Arctic pollution (2020) · cites this paper as Bauduin et al ., 2014
The paper’s introduction says Norilsk’s pollution is directly responsible for degradation and contamination of the surrounding environment. Its retrieval discussion reports SO₂ over about 165,000 km² but describes environmental influence as suggested, not measured habitat destruction. The cited passages do not establish that vast areas of taiga and tundra habitat on the Taimyr Peninsula were destroyed. (LLM, conf=0.85)
Experimental — accuracy not yet measuredSince the mid-20th century, continuous SO2 emissions from high-latitude mining, oil and shipping activities have affected biogeochemical cycles over central and eastern Siberia and across much of the circumpolar Arctic.
“Since the mid-20th century, continuous SO2 emissions from high-latitude mining, oil and shipping activities (Fig. S1; Table S9) have affected biogeochemical cycles not only over central and eastern Siberia (Shevchenko et al ., 2003), but also across much of the circumpolar Arctic (Hirdman et al ., 2010; Bauduin et al ., 2014; Panyushkina et al ., 2016).”
From Ecological and conceptual consequences of Arctic pollution (2020) · cites this paper as Bauduin et al., 2014
The paper’s introductory passage (page unavailable) says Norilsk’s smelters emit SO₂ and that pollution from the region contributes to Arctic air pollution. It does not establish effects on biogeochemical cycles across much of the circumpolar Arctic, or attribute such effects to oil and shipping emissions since the mid-20th century. (LLM, conf=0.83)
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Citations
Cites
Arctic Air Pollution: Origins and Impacts
Law, K. S., & Stohl, A. (2007) · Science · doi:10.1126/science.1137695 · Cited by 459
Zoning of Landscapes Exposed to Technogenic Emissions from the Norilsk Mining and Smelting Works
Zubareva, O. N., Skripal'shchikova, L. N., Greshilova, N. V., & Kharuk, V. I. (2003) · Russian Journal of Ecology · doi:10.1023/a:1027356316112 · Cited by 20 · cited 1×
“…responsible for the degradation and contamination of the surrounding environment [Vlasova et al., 1991; Blais et al., 1999; Tutubalina and Rees, 2001; Allen-Gil et al., 2003; Zubareva et al., 2003] and which contribute to the Arctic air pollution [Law and Stohl, 2007; Hirdman et al., 2010].”
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Cited by
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Ecological and conceptual consequences of Arctic pollution
Kirdyanov, A. V., Krusic, P. J., Shishov, V. V., Vaganov, E. A., Fertikov, A. I., Myglan, V. S., Barinov, V. V., Browse, J., Esper, J., Ilyin, V. A., et al. (2020) · Ecology Letters · doi:10.1111/ele.13611 · Cited by 60
Metadata
- Authors
- Bauduin, S., Clarisse, L., Clerbaux, C., Hurtmans, D., & Coheur, P.
- Affiliations
- Université Libre de Bruxelles (BE)
- Centre National de la Recherche Scientifique (FR)
- Corresponding author
- Bauduin, Sophie
- Venue
- Journal of Geophysical Research: Atmospheres
- Publisher
- American Geophysical Union (AGU)
- Published
- 2014-04-07
- Volume
- 119
- Issue
- 7
- Pages
- 4253-4263
- ISSN
- 0148-0227 (ISSN-L)
- 2169-897X
- 2169-8996
- OpenAlex
- W2062727408
- Cited by
- 52
- References
- 2
- Citations by year
- 2026: 3 · 2024: 5 · 2023: 9 · 2022: 4 · 2021: 3 · 2020: 4 · 2019: 3 · 2018: 2 · 2017: 4 · 2016: 7 · 2015: 4 · 2014: 4
- FWCI
- 4.21
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Journal of Geophysical Research Atmospheres (publishedVersion)
- HAL (submittedVersion, other-oa)
- Dépôt institutionnel de l'Université libre de Bruxelles (Université Libre de Bruxelles) (submittedVersion, other-oa)
- Topics
- Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric chemistry and aerosols
- Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric aerosols and clouds
- Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric and Environmental Gas Dynamics
- Keywords
- sulfur dioxide, Norilsk, IASI, boundary layer, anthropogenic pollution, sulfur dioxide emissions, temperature inversion, surface humidity, retrieval errors, box model, satellite remote sensing
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