The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Biomass burning dominates brown carbon absorption in the rural southeastern United States
Open accessAbstract
Brown carbon aerosol consists of light‐absorbing organic particulate matter with wavelength‐dependent absorption. Aerosol optical extinction, absorption, size distributions, and chemical composition were measured in rural Alabama during summer 2013. The field site was well located to examine sources of brown carbon aerosol, with influence by high biogenic organic aerosol concentrations, pollution from two nearby cities, and biomass burning aerosol. We report the optical closure between measured dry aerosol extinction at 365 nm and calculated extinction from composition and size distribution, showing agreement within experiment uncertainties. We find that aerosol optical extinction is dominated by scattering, with single‐scattering albedo values of 0.94 ± 0.02. Black carbon aerosol accounts for 91 ± 9% of the total carbonaceous aerosol absorption at 365 nm, while organic aerosol accounts for 9 ± 9%. The majority of brown carbon aerosol mass is associated with biomass burning, with smaller contributions from biogenically derived secondary organic aerosol.
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Cites
Bounding the role of black carbon in the climate system: A scientific assessment
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., et al. (2013) · Journal of Geophysical Research: Atmospheres · doi:10.1002/jgrd.50171 · Cited by 6,385
Light Absorption by Carbonaceous Particles: An Investigative Review
Bond, T. C., & Bergstrom, R. W. (2006) · Aerosol Science and Technology · doi:10.1080/02786820500421521 · Cited by 2,980
Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols
Andreae, M. O., & Gelencsér, A. (2006) · Atmospheric Chemistry and Physics · doi:10.5194/acp-6-3131-2006 · Cited by 2,006
Bones, D. L., Henricksen, D. K., Mang, S. A., Gonsior, M., Bateman, A. P., Nguyen, T. B., Cooper, W. J., & Nizkorodov, S. A. (2010) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2009jd012864 · Cited by 299
Cited by
Lee, B. H., Mohr, C., Lopez-Hilfiker, F. D., Lutz, A., Hallquist, M., Lee, L., Romer, P., Cohen, R. C., Iyer, S., Kurtén, T., et al. (2016) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1508108113 · Cited by 389
Self-citationMolecular Chemistry of Atmospheric Brown Carbon Inferred from a Nationwide Biomass Burning Event
Lin, P., Bluvshtein, N., Rudich, Y., Nizkorodov, S. A., Laskin, J., & Laskin, A. (2017) · Environmental Science & Technology · doi:10.1021/acs.est.7b02276 · Cited by 382
Photochemical processing of aqueous atmospheric brown carbon
Zhao, R., Lee, A. K. Y., Huang, L., Li, X., Yang, F., & Abbatt, J. P. D. (2015) · Atmospheric Chemistry and Physics · doi:10.5194/acp-15-6087-2015 · Cited by 373
Liu, X., Huey, L. G., Yokelson, R. J., Selimovic, V., Simpson, I. J., Müller, M., Jimenez, J. L., Campuzano‐Jost, P., Beyersdorf, A. J., Blake, D. R., et al. (2017) · Journal of Geophysical Research: Atmospheres · doi:10.1002/2016jd026315 · Cited by 308
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Metadata
- Authors
- Washenfelder, R. A., Attwood, A. R., Brock, C. A., Guo, H., Xu, L., Weber, R. J., Ng, N. L., Allen, H. M., Ayres, B. R., Baumann, K., Cohen, R. C., Draper, D. C., Duffey, K. C., Edgerton, E., Fry, J. L., Hu, W. W., Jimenez, J. L., Palm, B. B., Romer, P., Stone, E. A., Wooldridge, P. J., & Brown, S. S.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 2015-01-28
- Volume
- 42
- Issue
- 2
- Pages
- 653-664
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2136753478
- Cited by
- 284
- References
- 4
- FWCI
- 17.87
- Type
- journal article
- Language
- en
- Open access
- green
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- Washenfelder, R. A., Attwood, A. R., Brock, C. A., Guo, H., Xu, L., Weber, R. J., Ng, N. L., Allen, H. M., Ayres, B. R., Baumann, K., Cohen, R. C., Draper, D. C., Duffey, K. C., Edgerton, E., Fry, J. L., Hu, W. W., Jimenez, J. L., Palm, B. B., Romer, P., . . . Brown, S. S. (2015). Biomass burning dominates brown carbon absorption in the rural southeastern United States. Geophysical Research Letters. https://doi.org/10.1002/2014gl062444
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