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Thermosensitive Nanostructures Comprising Gold Nanoparticles Grafted with Block Copolymers
Abstract
Binary thermosensitive nanocomposites are fabricated by grafting block copolymers of poly(N‐isopropylacrylamide) and poly(methoxy‐oligo(ethylene glycol) methacrylate) onto gold nanoparticles through consecutive, surface‐initiated, atom‐transfer radical polymerization (ATRP). These Au@copolymer nanocomposites display a well‐defined core/shell nanostructure and have two thermosensitive points near 33 and 55 °C in an aqueous suspension corresponding to the thermally induced conformational transition of inner homopolymer segments and outer oligo(ethylene glycol)‐containing copolymer layer, respectively. Silver nanoparticles trapped within Au@copolymer nanocomposites with weakly crosslinked shells display thermally modulated catalytic activity as heterogeneous catalysts because of the thermosensitive collapse of the polymer layers.
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You, Y., Hong, C., Wang, W., Lu, W., & Pan, C. (2004) · Macromolecules · doi:10.1021/ma048444t · Cited by 151
Cited by
Barbey, R., Lavanant, L., Paripovic, D., Schüwer, N., Sugnaux, C., Tugulu, S., & Klok, H.-A. (2009) · Chemical Reviews · doi:10.1021/cr900045a · Cited by 1,753
Zoppe, J. O., Ataman, N. C., Mocny, P., Wang, J., Moraes, J., & Klok, H.-A. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00314 · Cited by 1,046
Morandi, G., Heath, L., & Thielemans, W. (2009) · Langmuir · doi:10.1021/la900452a · Cited by 405
Toward functional nanocomposites: taking the best of nanoparticles, polymers, and small molecules
Kao, J., Thorkelsson, K., Bai, P., Rancatore, B. J., & Xu, T. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35375j · Cited by 386
Zhu, M., Wang, C., Meng, D., & Diao, G. (2013) · J. Mater. Chem. A · doi:10.1039/c2ta00669c · Cited by 275
Metadata
- Authors
- Li, D., Cui, Y., Wang, K., He, Q., Yan, X., & Li, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2007-09-20
- Volume
- 17
- Issue
- 16
- Pages
- 3134-3140
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W1974867058
- Cited by
- 179
- References
- 1
- FWCI
- 6.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, D., Cui, Y., Wang, K., He, Q., Yan, X., & Li, J. (2007). Thermosensitive Nanostructures Comprising Gold Nanoparticles Grafted with Block Copolymers. Advanced Functional Materials. https://doi.org/10.1002/adfm.200700427
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
