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Graphene‐Based Nanoporous Materials Assembled by Mediation of Polyoxometalate Nanoparticles
Abstract
A kind of graphene‐based nanoporous material is prepared through assembling graphene sheets mediated through polyoxometalate nanoparticles. Owing to the strong interaction between graphene and polyoxometalate, 2D graphene sheets with honeycomb‐latticed carbon atoms could assemble into a porous structure, in which 3D polyoxometalate nanoparticles serve as the crosslinkers. Nitrogen and hydrogen sorption analysis reveal that the as‐prepared graphene‐based hybrid material possesses a specific surface area of 680 m 2 g−1 and a hydrogen uptake volume of 0.8−1.3 wt%. Infrared spectrometry is used to probe the electron density changes of polyoxometalate particle in the redox‐cycle and to verify the interaction between graphene and polyoxometalate. The as‐prepared graphene‐based materials are further characterized by Raman spectroscopy, X‐ray diffraction, scanning electron microscopy, and transmission electron microscopy.
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Cites
Scheuermann, G. M., Rumi, L., Steurer, P., Bannwarth, W., & Mülhaupt, R. (2009) · Journal of the American Chemical Society · doi:10.1021/ja901105a · Cited by 1,163
Cited by
Li, J.-S., Wang, Y., Liu, C.-H., Li, S.-L., Wang, Y.-G., Dong, L.-Z., Dai, Z.-H., Li, Y.-F., & Lan, Y.-Q. (2016) · Nature Communications · doi:10.1038/ncomms11204 · Cited by 990
Graphene-based materials: Synthesis and gas sorption, storage and separation
Gadipelli, S., & Guo, Z. X. (2015) · Progress in Materials Science · doi:10.1016/j.pmatsci.2014.10.004 · Cited by 734
Metadata
- Authors
- Zhou, D., & Han, B.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2010-07-02
- Volume
- 20
- Issue
- 16
- Pages
- 2717-2722
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2132214742
- Cited by
- 220
- References
- 1
- FWCI
- 5.56
- Type
- journal article
- Language
- en
- Open access
- closed
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