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High‐Performance Carbon‐LiMnPO4 Nanocomposite Cathode for Lithium Batteries
Abstract
A cathode material of an electrically conducting carbon‐LiMnPO 4 nanocomposite is synthesized by ultrasonic spray pyrolysis followed by ball milling. The effect of the carbon content on the physicochemical and electrochemical properties of this material is extensively studied. A LiMnPO 4 electrode with 30 wt% acetylene black (AB) carbon exhibits an excellent rate capability and good cycle life in cell tests at 55 and 25 °C. This electrode delivers a discharge capacity of 158 mAh g−1 at 1/20 C, 126 mAh g−1 at 1 C, and 107 mAh g−1 at 2 C rate, which are the highest capacities reported so far for this type of electrode. Transmission electron microscopy and Mn dissolution results confirm that the carbon particles surrounding the LiMnPO 4 protect the electrode from HF attack, and thus lead to a reduction of the Mn dissolution that usually occurs with this electrode. The improved electrochemical properties of the C‐LiMnPO 4 electrode are also verified by electrochemical impedance spectroscopy.
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Cited by
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Prospective materials and applications for Li secondary batteries
Jeong, G., Kim, Y.-U., Kim, H., Kim, Y.-J., & Sohn, H.-J. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00831a · Cited by 616
Recent advances in the research of polyanion-type cathode materials for Li-ion batteries
Gong, Z., & Yang, Y. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00713g · Cited by 549
LiMnPO4 – A next generation cathode material for lithium-ion batteries
Aravindan, V., Gnanaraj, J., Lee, Y.-S., & Madhavi, S. (2013) · Journal of Materials Chemistry A · doi:10.1039/c2ta01393b · Cited by 466
Reducing cobalt from lithium-ion batteries for the electric vehicle era
Ryu, H.-H., Sun, H. H., Myung, S.-T., Yoon, C. S., & Sun, Y.-K. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03581e · Cited by 331
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Metadata
- Authors
- Oh, S., Oh, S., Yoon, C., Scrosati, B., Amine, K., & Sun, Y.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2010-08-04
- Volume
- 20
- Issue
- 19
- Pages
- 3260-3265
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2012995907
- Cited by
- 396
- References
- 0
- FWCI
- 28.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Oh, S., Oh, S., Yoon, C., Scrosati, B., Amine, K., & Sun, Y. (2010). High‐Performance Carbon‐LiMnPO4 Nanocomposite Cathode for Lithium Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.201000469
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