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Phosphorous Pentasulfide as a Novel Additive for High‐Performance Lithium‐Sulfur Batteries
Abstract
Lithium‐sulfur (Li‐S) batteries suffer from rapid capacity decay and low energy efficiency because of the low solubility of lithium sulfide (Li 2 S) in organic solvents and the intrinsic polysulfide shuttle phenomenon. Here, a novel additive, phosphorus pentasulfide (P 2 S 5) in organic electrolyte, is reported to boost the cycling performance of Li‐S batteries. The function of the additive is two‐fold: 1) P 2 S 5 promotes the dissolution of Li 2 S and alleviates the loss of capacity caused by the precipitation of Li 2 S and 2) P 2 S 5 passivates the surface of lithium metal and therefore eliminates the polysulfide shuttle phenomenon. A Li‐S test cell demonstrates a high reversible capacity of 900–1350 mAh g−1 and a high coulombic efficiency of ≥90% for at least 40 stable cycles at 0.1 C.
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Cites
Lithium Batteries: Status, Prospects and Future
Scrosati, B., & Garche, J. (2010) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.11.048 · Cited by 5,153
Cited by
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Wang, Z., Dong, Y., Li, H., Zhao, Z., Bin Wu, H., Hao, C., Liu, S., Qiu, J., & Lou, X. W. (2014) · Nature Communications · doi:10.1038/ncomms6002 · Cited by 1,059
Zhang, H., Eshetu, G. G., Judez, X., Li, C., Rodriguez‐Martínez, L. M., & Armand, M. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712702 · Cited by 774
From lithium to sodium: Cell chemistry of room temperature sodium–air and sodium–sulfur batteries
Adelhelm, P., Hartmann, P., Bender, C. L., Busche, M., Eufinger, C., & Janek, J. (2015) · Beilstein Journal of Nanotechnology · doi:10.3762/bjnano.6.105 · Cited by 478
Investigations of lithium–sulfur batteries using electrochemical impedance spectroscopy
Cañas, N. A., Hirose, K., Pascucci, B., Wagner, N., Friedrich, K. A., & Hiesgen, R. (2013) · Electrochimica Acta · doi:10.1016/j.electacta.2013.02.101 · Cited by 415
Metadata
- Authors
- Lin, Z., Liu, Z., Fu, W., Dudney, N. J., & Liang, C.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2012-06-14
- Volume
- 23
- Issue
- 8
- Pages
- 1064-1069
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2039693575
- Cited by
- 450
- References
- 1
- FWCI
- 21.57
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lin, Z., Liu, Z., Fu, W., Dudney, N. J., & Liang, C. (2013). Phosphorous Pentasulfide as a Novel Additive for High‐Performance Lithium‐Sulfur Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.201200696
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