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Edge‐Fluorinated Graphene Nanoplatelets as High Performance Electrodes for Dye‐Sensitized Solar Cells and Lithium Ion Batteries
Abstract
Edge‐selectively fluorinated graphene nanoplatelets (FGnPs) are prepared by mechanochemically driven reaction between fluorine gas (20 vol% in argon) and activated carbon species from graphitic C–C bonds unzipped by high‐speed stainless steel balls with a high kinetic energy. The fluorination at edges of the unzipped graphene nanoplatelets (GnPs) is confirmed by various analytical techniques while the content of fluorine in FGnPs is determined to be 3.0 and 3.4 at% by X‐ray photoelectron spectroscopy and energy‐dispersive X‐ray spectroscopy, respectively. Because of the large difference in electronegativity between carbon (χ = 2.55) and fluorine (χ = 3.98) and the strong C–F bond, the edge‐fluorination of GnPs can provide the maximized charge polarization with an enhanced chemical stability. Thus, electrodes based on the resultant FGnPs demonstrate superb electrochemical performance with excellent stability/cycle life in dye‐sensitized solar cells (FF: 71.5%; Jsc: 14.44 mA cm−2; Voc: 970 mV; PCE: 10.01%) and lithium ion batteries (650.3 mA h g−1 at 0.5 C, charge retention of 76.6% after 500 cycles).
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Cites
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Ageing mechanisms in lithium-ion batteries
Vetter, J., Novák, P., Wagner, M. R., Veit, C., Möller, K.-C., Besenhard, J. O., Winter, M., Wohlfahrt-Mehrens, M., Vogler, C., & Hammouche, A. (2005) · Journal of Power Sources · doi:10.1016/j.jpowsour.2005.01.006 · Cited by 3,987
Cited by
Two‐Dimensional Fluorinated Graphene: Synthesis, Structures, Properties and Applications
Feng, W., Long, P., Feng, Y., & Li, Y. (2016) · Advanced Science · doi:10.1002/advs.201500413 · Cited by 640
Heteroatom-doped carbon-based materials for lithium and sodium ion batteries
Yuan, Y., Chen, Z., Yu, H., Zhang, X., Liu, T., Xia, M., Zheng, R., Shui, M., & Shu, J. (2020) · Energy Storage Materials · doi:10.1016/j.ensm.2020.07.027 · Cited by 455
Xing, Z., Ju, Z., Zhao, Y., Wan, J., Zhu, Y., Qiang, Y., & Qian, Y. (2016) · Scientific Reports · doi:10.1038/srep26146 · Cited by 435
Carbon-based functional nanomaterials: Preparation, properties and applications
Li, Z., Wang, L., Li, Y., Feng, Y., & Feng, W. (2019) · Composites Science and Technology · doi:10.1016/j.compscitech.2019.04.028 · Cited by 384
Chemistry, properties, and applications of fluorographene
Chronopoulos, D. D., Bakandritsos, A., Pykal, M., Zbořil, R., & Otyepka, M. (2017) · Applied Materials Today · doi:10.1016/j.apmt.2017.05.004 · Cited by 284
Metadata
- Authors
- Jeon, I., Ju, M. J., Xu, J., Choi, H., Seo, J., Kim, M., Choi, I. T., Kim, H. M., Kim, J. C., Lee, J., Liu, H. K., Kim, H. K., Dou, S., Dai, L., & Baek, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2015-01-08
- Volume
- 25
- Issue
- 8
- Pages
- 1170-1179
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2137490554
- Cited by
- 216
- References
- 2
- FWCI
- 11.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jeon, I., Ju, M. J., Xu, J., Choi, H., Seo, J., Kim, M., Choi, I. T., Kim, H. M., Kim, J. C., Lee, J., Liu, H. K., Kim, H. K., Dou, S., Dai, L., & Baek, J. (2015). Edge‐Fluorinated Graphene Nanoplatelets as High Performance Electrodes for Dye‐Sensitized Solar Cells and Lithium Ion Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.201403836
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