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MoS2/Si Heterojunction with Vertically Standing Layered Structure for Ultrafast, High‐Detectivity, Self‐Driven Visible–Near Infrared Photodetectors

Wang, Liu, Jie, Jiansheng, Shao, Zhibin, Zhang, Qing, Zhang, Xiaohong, Wang, Yuming, Sun, Zheng, Lee, Shuit‐Tong·2015·Advanced Functional Materials

Abstract

As an interesting layered material, molybdenum disulfide (MoS 2) has been extensively studied in recent years due to its exciting properties. However, the applications of MoS 2 in optoelectronic devices are impeded by the lack of high‐quality p–n junction, low light absorption for mono‐/multilayers, and the difficulty for large‐scale monolayer growth. Here, it is demonstrated that MoS 2 films with vertically standing layered structure can be deposited on silicon substrate with a scalable sputtering method, forming the heterojunction‐type photodetectors. Molecular layers of the MoS 2 films are perpendicular to the substrate, offering high‐speed paths for the separation and transportation of photo‐generated carriers. Owing to the strong light absorption of the relatively thick MoS 2 film and the unique vertically standing layered structure, MoS 2/Si heterojunction photodetectors with unprecedented performance are actualized. The self‐driven MoS 2/Si heterojunction photodetector is sensitive to a broadband wavelength from visible light to near‐infrared light, showing an extremely high detectivity up to ≈10 13 Jones (Jones = cm Hz 1/2 W−1), and an ultrafast response speed of ≈3 μs. The performance is significantly better than the photodetectors based on mono‐/multilayer MoS 2 nanosheets. Additionally, the MoS 2/Si photodetectors exhibit excellent stability in air for a month. This work unveils the great potential of MoS 2/Si heterojunction for optoelectronic applications.

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Metadata

Authors
Wang, L., Jie, J., Shao, Z., Zhang, Q., Zhang, X., Wang, Y., Sun, Z., & Lee, S.
Venue
Advanced Functional Materials
Publisher
Wiley
Published
2015-03-30
Volume
25
Issue
19
Pages
2910-2919
ISSN
  • 1616-301X (ISSN-L)
  • 1616-3028
OpenAlex
W2030927935
Cited by
684
References
8
FWCI
21.85
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: MoS2/Si Heterojunction with Vertically Standing Layered Structure for Ultrafast, High‐Detectivity, Self‐Driven Visible–Near Infrared Photodetectors. https://app.cochat.ai/papers/10.1002/adfm.201500216
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Wang, L., Jie, J., Shao, Z., Zhang, Q., Zhang, X., Wang, Y., Sun, Z., & Lee, S. (2015). MoS2/Si Heterojunction with Vertically Standing Layered Structure for Ultrafast, High‐Detectivity, Self‐Driven Visible–Near Infrared Photodetectors. Advanced Functional Materials. https://doi.org/10.1002/adfm.201500216

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