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High‐Performance Inverted Planar Heterojunction Perovskite Solar Cells Based on Lead Acetate Precursor with Efficiency Exceeding 18%
Open accessAbstract
Organic–inorganic lead halide perovskites are emerging materials for the next‐generation photovoltaics. Lead halides are the most commonly used lead precursors for perovskite active layers. Recently, lead acetate (Pb(Ac)2) has shown its superiority as the potential replacement for traditional lead halides. Here, we demonstrate a strategy to improve the efficiency for the perovskite solar cell based on lead acetate precursor. We utilized methylammonium bromide as an additive in the Pb(Ac)2 and methylammonium iodide precursor solution, resulting in uniform, compact and pinhole‐free perovskite films. We observed enhanced charge carrier extraction between the perovskite layer and charge collection layers and delivered a champion power conversion efficiency of 18.3% with a stabilized output efficiency of 17.6% at the maximum power point. The optimized devices also exhibited negligible current density–voltage (J–V) hysteresis under the scanning conditions.
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Cites
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Cited by
Causes and Solutions of Recombination in Perovskite Solar Cells
Chen, J., & Park, N. (2019) · Advanced Materials · doi:10.1002/adma.201803019 · Cited by 733
Synthetic Approaches for Halide Perovskite Thin Films
Dunlap-Shohl, W. A., Zhou, Y., Padture, N. P., & Mitzi, D. B. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00318 · Cited by 631
All‐Carbon‐Electrode‐Based Endurable Flexible Perovskite Solar Cells
Luo, Q., Ma, H., Hou, Q., Li, Y., Ren, J., Dai, X., Yao, Z., Zhou, Y., Xiang, L., Du, H., et al. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201706777 · Cited by 346
Efficiency progress of inverted perovskite solar cells
Lin, X., Cui, D., Luo, X., Zhang, C., Han, Q., Wang, Y., & Han, L. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02017f · Cited by 346
Metadata
- Authors
- Zhao, L., Luo, D., Wu, J., Hu, Q., Zhang, W., Chen, K., Liu, T., Liu, Y., Zhang, Y., Liu, F., Russell, T. P., Snaith, H. J., Zhu, R., & Gong, Q.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2016-04-13
- Volume
- 26
- Issue
- 20
- Pages
- 3508-3514
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2337959965
- Cited by
- 191
- References
- 2
- FWCI
- 18.14
- Type
- journal article
- Language
- en
- Open access
- green
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- Zhao, L., Luo, D., Wu, J., Hu, Q., Zhang, W., Chen, K., Liu, T., Liu, Y., Zhang, Y., Liu, F., Russell, T. P., Snaith, H. J., Zhu, R., & Gong, Q. (2016). High‐Performance Inverted Planar Heterojunction Perovskite Solar Cells Based on Lead Acetate Precursor with Efficiency Exceeding 18%. Advanced Functional Materials. https://doi.org/10.1002/adfm.201601175
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