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Black Phosphorus and Polymeric Carbon Nitride Heterostructure for Photoinduced Molecular Oxygen Activation
Abstract
Metal‐free heterostructure photocatalysts composed of black phosphorus (BP) and polymeric carbon nitride (CN) are successfully synthesized via a one‐step liquid exfoliation method assisted by sonication. The combination of BP with CN strengthens the visible‐light harvesting ability, facilitates the charge separation in the photocatalytic process, and renders promoted activity of photoinduced molecular oxygen activation, such as superoxide radicals (·O 2−) evolution and H 2 O 2 production. This work highlights that coupling semiconductors with well‐matched band levels provide a flexible route to enhance the performance of photocatalysts for producing reactive oxygen species, and gives ideas for the design of highly active and metal‐free materials toward sustainable solar‐to‐chemical energy conversion and environmental remediation.
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Cui, Y., Ding, Z., Liu, P., Antonietti, M., Fu, X., & Wang, X. (2012) · Phys. Chem. Chem. Phys. · doi:10.1039/c1cp22820j · Cited by 585
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Photocatalytic H2O2 production Systems: Design strategies and environmental applications
Chen, Z., Yao, D., Chu, C., & Mao, S. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.138489 · Cited by 482
Enhanced Photocatalytic H2O2 Production over Carbon Nitride by Doping and Defect Engineering
Wu, S., Yu, H., Chen, S., & Quan, X. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03359 · Cited by 466
Yang, Y., Zeng, G., Huang, D., Zhang, C., He, D., Zhou, C., Wang, W., Xiong, W., Li, X., Li, B., et al. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.118970 · Cited by 412
Wang, W., Niu, Q., Zeng, G., Zhang, C., Huang, D., Shao, B., Zhou, C., Yang, Y., Liu, Y., Guo, H., et al. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119051 · Cited by 409
Liu, L., Gao, M.-Y., Yang, H., Wang, X., Li, X., & Cooper, A. I. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.1c09979 · Cited by 394
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Metadata
- Authors
- Zheng, Y., Yu, Z., Ou, H., Asiri, A. M., Chen, Y., & Wang, X.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2018-01-08
- Volume
- 28
- Issue
- 10
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2783284181
- Cited by
- 462
- References
- 1
- FWCI
- 14.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zheng, Y., Yu, Z., Ou, H., Asiri, A. M., Chen, Y., & Wang, X. (2018). Black Phosphorus and Polymeric Carbon Nitride Heterostructure for Photoinduced Molecular Oxygen Activation. Advanced Functional Materials. https://doi.org/10.1002/adfm.201705407
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