The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Atomic Pd on Graphdiyne/Graphene Heterostructure as Efficient Catalyst for Aromatic Nitroreduction
Abstract
With the maximum atom‐utilization efficiency, single atom catalysts (SACs) have attracted great research interest in catalysis science recently. To address the following key challenges for the further development of SACs: i) how to stabilize and avoid the aggregation of SACs, ii) how to enhance the specific surface area and conductivity of supports, and iii) how to achieve scalable mass production with low cost, a SAC consisting of single Pd atoms anchored on well‐designed graphdiyne/graphene (GDY/G) heterostructure (Pd 1/GDY/G) is synthesized. Pd 1/GDY/G exhibits high catalytic performance, as demonstrated by the reduction reaction of 4‐nitrophenol. Furthermore, density functional theory calculation indicates that graphene in the GDY/G heterostructure plays a key role in the enhancement of catalytic efficiency owing to the electron transfer process, deriving from the gap between the Fermi level of graphene and the conduction band minimum of GDY. The GDY/G heterostructure is a promising support for the preparation of extremely efficient and stable SACs, which can be used in a broad range of future industrial reactions.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
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Atomic cobalt on nitrogen-doped graphene for hydrogen generation
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Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
Xue, Y., Huang, B., Yi, Y., Guo, Y., Zuo, Z., Li, Y., Jia, Z., Liu, H., & Li, Y. (2018) · Nature Communications · doi:10.1038/s41467-018-03896-4 · Cited by 1,011
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
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Self-citationCharge-Transfer Induced High Efficient Hydrogen Evolution of MoS2/graphene Cocatalyst
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Cited by
Single-Atom Catalysts across the Periodic Table
Kaiser, S. K., Chen, Z., Faust Akl, D., Mitchell, S., & Pérez-Ramírez, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00576 · Cited by 1,367
2D graphdiyne: An emerging carbon material
Fang, Y., Liu, Y., Qi, L., Xue, Y., & Li, Y. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00592h · Cited by 520
Zhu, P., Xiong, X., & Wang, D. (2022) · Nano Research · doi:10.1007/s12274-022-4265-y · Cited by 375
Supports promote single-atom catalysts toward advanced electrocatalysis
Xu, H., Zhao, Y., Wang, Q., He, G., & Chen, H. (2022) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.214261 · Cited by 363
Two-Dimensional Carbon Graphdiyne: Advances in Fundamental and Application Research
Zheng, X., Chen, S., Li, J., Wu, H., Zhang, C., Zhang, D., Chen, X., Gao, Y., He, F., Hui, L., et al. (2023) · ACS Nano · doi:10.1021/acsnano.3c03849 · Cited by 283
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Metadata
- Authors
- Li, J., Zhong, L., Tong, L., Yu, Y., Liu, Q., Zhang, S., Yin, C., Qiao, L., Li, S., Si, R., & Zhang, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2019-08-16
- Volume
- 29
- Issue
- 43
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2967873079
- Cited by
- 170
- References
- 8
- FWCI
- 7.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, J., Zhong, L., Tong, L., Yu, Y., Liu, Q., Zhang, S., Yin, C., Qiao, L., Li, S., Si, R., & Zhang, J. (2019). Atomic Pd on Graphdiyne/Graphene Heterostructure as Efficient Catalyst for Aromatic Nitroreduction. Advanced Functional Materials. https://doi.org/10.1002/adfm.201905423
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