The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Achieving Both High Voltage and High Capacity in Aqueous Zinc‐Ion Battery for Record High Energy Density
Open accessAbstract
In this work, a high‐voltage output and long‐lifespan zinc/vanadium oxide bronze battery using a Co 0.247 V 2 O 5⋅0.944H 2 O nanobelt is developed. The high crystal architecture could enable fast and reversible Zn 2+ intercalation/deintercalation at highly operational voltages. The developed battery exhibits a high voltage of 1.7 V and delivers a high capacity of 432 mAh g−1 at 0.1 A g−1. The capacity at voltages above 1.0 V reaches 227 mAh g−1, which is 52.54% of the total capacity and higher than the values of all previously reported Zn/vanadium oxide batteries. Further study reveals that, compared with the pristine vanadium oxide bronze, the absorption energy for Zn 2+ increases from 1.85 to 2.24 eV by cobalt ion intercalation. Furthermore, it also shows a high rate capability (163 mAh g−1 even at 10 A g−1) and extraordinary lifespan over 7500 cycles, with a capacity retention of 90.26%. These performances far exceed those for all reported zinc/vanadium oxide bronze batteries. Subsequently, a nondrying and antifreezing tough flexible battery with a high energy density of 432 Wh kg−1 at 0.1 A g−1 is constructed, and it reveals excellent drying and freezing tolerance. This research represents a substantial advancement in vanadium materials for various battery applications, achieving both a high discharge voltage and high capacity.
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Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
Chen, M., Chen, J., Zhou, W., Han, X., Yao, Y., & Wong, C. (2021) · Advanced Materials · doi:10.1002/adma.202007559 · Cited by 428
Wang, X., Xi, B., Ma, X., Feng, Z., Jia, Y., Feng, J., Qian, Y., & Xiong, S. (2020) · Nano Letters · doi:10.1021/acs.nanolett.0c00732 · Cited by 331
Rechargeable aqueous zinc-ion batteries: Mechanism, design strategies and future perspectives
Liu, H., Wang, J.-G., You, Z., Wei, C., Kang, F., & Wei, B. (2021) · Materials Today · doi:10.1016/j.mattod.2020.08.021 · Cited by 282
Metadata
- Authors
- Ma, L., Li, N., Long, C., Dong, B., Fang, D., Liu, Z., Zhao, Y., Li, X., Fan, J., Chen, S., Zhang, S., & Zhi, C.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2019-09-17
- Volume
- 29
- Issue
- 46
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2974428365
- Cited by
- 415
- References
- 1
- FWCI
- 20.27
- Type
- journal article
- Language
- en
- Open access
- green
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- Ma, L., Li, N., Long, C., Dong, B., Fang, D., Liu, Z., Zhao, Y., Li, X., Fan, J., Chen, S., Zhang, S., & Zhi, C. (2019). Achieving Both High Voltage and High Capacity in Aqueous Zinc‐Ion Battery for Record High Energy Density. Advanced Functional Materials. https://doi.org/10.1002/adfm.201906142
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