The DOI matches its Crossref record; 35 of the 35 references it cites were found in a registry or an index.
3D Porous Oxidation‐Resistant MXene/Graphene Architectures Induced by In Situ Zinc Template toward High‐Performance Supercapacitors
Abstract
2D MXene materials have attracted intensive attention in energy storage application. However, MXene usually undergoes serious face‐to‐face restacking and inferior stability, significantly preventing its further commercial application. Herein, to suppress the oxidation and self‐restacking of MXene, an efficient and fast self‐assembly route to prepare a 3D porous oxidation‐resistant MXene/graphene (PMG) composite with the assistance of an in situ sacrificial metallic zinc template is demonstrated. The self‐assembled 3D porous architecture can effectively prevent the oxidation of MXene layers with no evident variation in electrical conductivity in air at room temperature after two months, guaranteeing outstanding electrical conductivity and abundant electrochemical active sites accessible to electrolyte ions. Consequently, the PMG‐5 electrode possesses a striking specific capacitance of 393 F g−1, superb rate performance (32.7% at 10 V s−1), and outstanding cycling stability. Furthermore, the as‐assembled asymmetric supercapacitor possesses a pronounced energy density of 50.8 Wh kg−1 and remarkable cycling stability with a 4.3% deterioration of specific capacitance after 10 000 cycles. This work paves a new avenue to solve the two long‐standing significant challenges of MXene in the future.
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Cites
2D metal carbides and nitrides (MXenes) for energy storage
Anasori, B., Lukatskaya, M. R., & Gogotsi, Y. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.98 · Cited by 7,440
Cation Intercalation and High Volumetric Capacitance of Two-Dimensional Titanium Carbide
Lukatskaya, M. R., Mashtalir, O., Ren, C. E., Dall’Agnese, Y., Rozier, P., Taberna, P. L., Naguib, M., Simon, P., Barsoum, M. W., & Gogotsi, Y. (2013) · Science · doi:10.1126/science.1241488 · Cited by 4,320
Ultra-high-rate pseudocapacitive energy storage in two-dimensional transition metal carbides
Lukatskaya, M. R., Kota, S., Lin, Z., Zhao, M.-Q., Shpigel, N., Levi, M. D., Halim, J., Taberna, P.-L., Barsoum, M. W., Simon, P., et al. (2017) · Nature Energy · doi:10.1038/nenergy.2017.105 · Cited by 2,335
Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance
Yan, J., Ren, C. E., Maleski, K., Hatter, C. B., Anasori, B., Urbankowski, P., Sarycheva, A., & Gogotsi, Y. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201701264 · Cited by 1,883
Self-citationScalable Manufacturing of Free‐Standing, Strong Ti3C2Tx MXene Films with Outstanding Conductivity
Zhang, J., Kong, N., Uzun, S., Levitt, A., Seyedin, S., Lynch, P. A., Qin, S., Han, M., Yang, W., Liu, J., et al. (2020) · Advanced Materials · doi:10.1002/adma.202001093 · Cited by 972
Zhao, S., Zhang, H.-B., Luo, J.-Q., Wang, Q.-W., Xu, B., Hong, S., & Yu, Z.-Z. (2018) · ACS Nano · doi:10.1021/acsnano.8b05739 · Cited by 893
Self-citationLi, X., Yin, X., Song, C., Han, M., Xu, H., Duan, W., Cheng, L., & Zhang, L. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201803938 · Cited by 716
Wang, H., Wu, Y., Yuan, X., Zeng, G., Zhou, J., Wang, X., & Chew, J. W. (2018) · Advanced Materials · doi:10.1002/adma.201704561 · Cited by 634
Fast Gelation of Ti3C2Tx MXene Initiated by Metal Ions
Deng, Y., Shang, T., Wu, Z., Tao, Y., Luo, C., Liang, J., Han, D., Lyu, R., Qi, C., Lv, W., et al. (2019) · Advanced Materials · doi:10.1002/adma.201902432 · Cited by 602
3D Macroscopic Architectures from Self‐Assembled MXene Hydrogels
Shang, T., Lin, Z., Qi, C., Liu, X., Li, P., Tao, Y., Wu, Z., Li, D., Simon, P., & Yang, Q. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201903960 · Cited by 506
Cited by
Shaikh, N. S., Ubale, S. B., Mane, V. J., Shaikh, J. S., Lokhande, V. C., Praserthdam, S., Lokhande, C. D., & Kanjanaboos, P. (2022) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2021.161998 · Cited by 253
Yang, Y., Huang, X., Sheng, C., Pan, Y., Huang, Y., & Wang, X. (2022) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2022.165908 · Cited by 68
Metadata
- Authors
- Yang, X., Wang, Q., Zhu, K., Ye, K., Wang, G., Cao, D., & Yan, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2021-03-12
- Volume
- 31
- Issue
- 20
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3136529912
- Cited by
- 308
- References
- 35
- FWCI
- 16.56
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, X., Wang, Q., Zhu, K., Ye, K., Wang, G., Cao, D., & Yan, J. (2021). 3D Porous Oxidation‐Resistant MXene/Graphene Architectures Induced by In Situ Zinc Template toward High‐Performance Supercapacitors. Advanced Functional Materials. https://doi.org/10.1002/adfm.202101087
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