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Single‐Atom Bi Alloyed Pd Metallene for Nitrate Electroreduction to Ammonia
Abstract
Electrochemical reduction of nitrate to ammonia (NO 3 RR) holds a great promise for attaining both NH 3 electrosynthesis and wastewater purification. Herein, single‐atom Bi alloyed Pd metallene (Bi 1 Pd) is reported as a highly effective NO 3 RR catalyst, showing a near 100% NH 3‐Faradaic efficiency with the corresponding NH 3 yield of 33.8 mg h−1 cm−2 at −0.6 V versus RHE, surpassing those of almost all ever reported NO 3 RR catalysts. In‐depth theoretical and operando spectroscopic investigations unveil that single‐atom Bi electronically couples with its neighboring Pd atoms to synergistically activate NO 3− and destabilize *NO on Bi 1 Pd, leading to the reduced energy barrier of the potential‐determining step (*NO→*NOH) and enhanced protonation energetics of NO 3−‐to‐NH 3 pathway.
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Citations
Cites
Metallenes as functional materials in electrocatalysis
Prabhu, P., & Lee, J.-M. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01041c · Cited by 427
Cited by
Fan, X., Chen, W., Xie, L., Liu, X., Ding, Y., Zhang, L., Tang, M., Liao, Y., Yang, Q., Fu, X., et al. (2024) · Advanced Materials · doi:10.1002/adma.202313179 · Cited by 89
Metadata
- Authors
- Chen, K., Ma, Z., Li, X., Kang, J., Ma, D., & Chu, K.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2023-01-15
- Volume
- 33
- Issue
- 12
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W4319835168
- Cited by
- 351
- References
- 1
- FWCI
- 16.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, K., Ma, Z., Li, X., Kang, J., Ma, D., & Chu, K. (2023). Single‐Atom Bi Alloyed Pd Metallene for Nitrate Electroreduction to Ammonia. Advanced Functional Materials. https://doi.org/10.1002/adfm.202209890
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