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n‐Type Building Blocks for Organic Electronics: A Homologous Family of Fluorocarbon‐Substituted Thiophene Oligomers with High Carrier Mobility
Abstract
A substantial enhancement of thermal stability, volatility, and electron affinity, switching the semiconducting behavior from p‐ to n‐type, is achieved by fluoroalkyl substitution of thiophene oligomers (see Figure). When this novel series is compared with the fluorine‐free analogues, trends in molecular packing, optical absorption, HOMO–LUMO gap, and π–π interactions are found to be strikingly similar.
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Citations
Cited by
Charge Carrier Transporting Molecular Materials and Their Applications in Devices
Shirota, Y., & Kageyama, H. (2007) · Chemical Reviews · doi:10.1021/cr050143+ · Cited by 1,756
Electron Transport Materials for Organic Light-Emitting Diodes
Kulkarni, A. P., Tonzola, C. J., Babel, A., & Jenekhe, S. A. (2004) · Chemistry of Materials · doi:10.1021/cm049473l · Cited by 1,624
Semiconductors for organic transistors
Facchetti, A. (2007) · Materials Today · doi:10.1016/s1369-7021(07)70017-2 · Cited by 874
Self-citationJones, B. A., Ahrens, M. J., Yoon, M., Facchetti, A., Marks, T. J., & Wasielewski, M. R. (2004) · Angewandte Chemie International Edition · doi:10.1002/anie.200461324 · Cited by 871
Self-citationOrganic thin film transistors: From theory to real devices
Horowitz, G. (2004) · Journal of Materials Research · doi:10.1557/jmr.2004.0266 · Cited by 852
Metadata
- Authors
- Facchetti, A., Mushrush, M., Katz, H. E., & Marks, T. J.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2003-01-03
- Volume
- 15
- Issue
- 1
- Pages
- 33-38
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2056658112
- Cited by
- 325
- References
- 0
- FWCI
- 30.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Facchetti, A., Mushrush, M., Katz, H. E., & Marks, T. J. (2003). n‐Type Building Blocks for Organic Electronics: A Homologous Family of Fluorocarbon‐Substituted Thiophene Oligomers with High Carrier Mobility. Advanced Materials. https://doi.org/10.1002/adma.200390003
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