The DOI matches its Crossref record; 23 of the 23 references it cites were found in a registry or an index.
Infrared Quantum Dots
Abstract
Colloidal nanocrystals are quantum‐size‐effect tunable; offer an abundance of available surface area for electronic and chemical interactions; and are processible from organic or aqueous solution onto substrates rigid or flexible, smooth or rough, flat or curved, inorganic or organic (including biological), crystalline or amorphous, conducting, semiconducting, or insulating. With the benefit of over a decade's progress in visible‐light‐emitting colloidal‐quantum‐dot synthesis, physical chemistry, and devices, significant progress has recently been made in infrared‐active colloidal quantum dots and devices. This progress report summarizes the state‐of‐the‐art in infrared colloidal quantum dots, with an emphasis on applications and devices. The applications of interest surveyed include monolithic integration of fiber‐optic and free‐space‐communications photonic components with electronic substrates such as silicon and glass; in‐vivo biological tagging in infrared spectral bands in which living tissue is optically penetrable to a depth of 5–10 cm; solar and thermal photovoltaics for energy conversion; and infrared sensing and imaging based on non‐visible, including thermal, signatures. The synthesis and properties of quantum dots are first reviewed: photoluminescence quantum efficiencies greater than 50 % are achievable in solution, and stable luminescent dots are available in organic and aqueous solvents. Electroluminescent devices based on solution processing have been reported with external quantum efficiencies approaching 1 %. Photoconductive devices have been realized with 3 % internal quantum efficiencies, and a photovoltaic effect was recently observed. Electro‐optic modulation achieved by either field‐ or charge‐induced modification of the rate of optical absorption has been demonstrated based both on interband and intersubband (intraband) transitions. Optical gain from these processible materials with a threshold of 1 mJ cm–2 and an optical net modal gain coefficient of 260 ± 20 cm–1 have been reported.
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Cites
In vivo cancer targeting and imaging with semiconductor quantum dots
Gao, X., Cui, Y., Levenson, R. M., Chung, L. W. K., & Nie, S. (2004) · Nature Biotechnology · doi:10.1038/nbt994 · Cited by 4,772
Optical gain in silicon nanocrystals
Pavesi, L., Dal Negro, L., Mazzoleni, C., Franzò, G., & Priolo, F. (2000) · Nature · doi:10.1038/35044012 · Cited by 2,315
Near-infrared fluorescent type II quantum dots for sentinel lymph node mapping
Kim, S., Lim, Y. T., Soltesz, E. G., De Grand, A. M., Lee, J., Nakayama, A., Parker, J. A., Mihaljevic, T., Laurence, R. G., Dor, D. M., et al. (2004) · Nature Biotechnology · doi:10.1038/nbt920 · Cited by 2,087
Fluorescence intermittency in single cadmium selenide nanocrystals
Nirmal, M., Dabbousi, B. O., Bawendi, M. G., Macklin, J. J., Trautman, J. K., Harris, T. D., & Brus, L. E. (1996) · Nature · doi:10.1038/383802a0 · Cited by 2,028
Solution-processed PbS quantum dot infrared photodetectors and photovoltaics
McDonald, S. A., Konstantatos, G., Zhang, S., Cyr, P. W., Klem, E. J. D., Levina, L., & Sargent, E. H. (2005) · Nature Materials · doi:10.1038/nmat1299 · Cited by 2,006
Hines, M. A., & Scholes, G. D. (2003) · Advanced Materials · doi:10.1002/adma.200305395 · Cited by 1,827
Quantization of Multiparticle Auger Rates in Semiconductor Quantum Dots
Klimov, V. I., Mikhailovsky, A. A., McBranch, D. W., Leatherdale, C. A., & Bawendi, M. G. (2000) · Science · doi:10.1126/science.287.5455.1011 · Cited by 1,521
Efficient Near-Infrared Polymer Nanocrystal Light-Emitting Diodes
Tessler, N., Medvedev, V., Kazes, M., Kan, S., & Banin, U. (2002) · Science · doi:10.1126/science.1068153 · Cited by 1,361
Lead Salt Quantum Dots: the Limit of Strong Quantum Confinement
Wise, F. W. (2000) · Accounts of Chemical Research · doi:10.1021/ar970220q · Cited by 1,182
Long-range resonance transfer of electronic excitations in close-packed CdSe quantum-dot solids
Kagan, C. R., Murray, C. B., & Bawendi, M. G. (1996) · Physical Review B · doi:10.1103/physrevb.54.8633 · Cited by 744
Crooker, S. A., Hollingsworth, J. A., Tretiak, S., & Klimov, V. I. (2002) · Physical Review Letters · doi:10.1103/physrevlett.89.186802 · Cited by 680
Selection of Quantum Dot Wavelengths for Biomedical Assays and Imaging
Lim, Y. T., Kim, S., Nakayama, A., Stott, N. E., Bawendi, M. G., & Frangioni, J. V. (2003) · Molecular Imaging · doi:10.1162/15353500200302163 · Cited by 559
Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well
Achermann, M., Petruska, M. A., Kos, S., Smith, D. L., Koleske, D. D., & Klimov, V. I. (2004) · Nature · doi:10.1038/nature02571 · Cited by 550
Steckel, J. S., Coe‐Sullivan, S., Bulović, V., & Bawendi, M. G. (2003) · Advanced Materials · doi:10.1002/adma.200305449 · Cited by 416
Bakueva, L., Musikhin, S., Hines, M. A., Chang, T.-W. F., Tzolov, M., Scholes, G. D., & Sargent, E. H. (2003) · Applied Physics Letters · doi:10.1063/1.1570940 · Cited by 372
Tunable Near-Infrared Optical Gain and Amplified Spontaneous Emission Using PbSe Nanocrystals
Schaller, R. D., Petruska, M. A., & Klimov, V. I. (2003) · The Journal of Physical Chemistry B · doi:10.1021/jp0311660 · Cited by 321
PbS Quantum Dots with Stable Efficient Luminescence in the Near‐IR Spectral Range
Bakueva, L., Gorelikov, I., Musikhin, S., Zhao, X. S., Sargent, E. H., & Kumacheva, E. (2004) · Advanced Materials · doi:10.1002/adma.200306458 · Cited by 229
McDonald, S. A., Cyr, P. W., Levina, L., & Sargent, E. H. (2004) · Applied Physics Letters · doi:10.1063/1.1792380 · Cited by 163
Sukhovatkin, V., Musikhin, S. F., Gorelikov, I., Cauchi, S., Bakueva, L., Kumacheva, E., & Sargent, E. H. (2005) · Optics Letters · doi:10.1364/ol.30.000171 · Cited by 100
Efficient excitation transfer from polymer to nanocrystals
Chang, T.-W. F., Musikhin, S. F., Bakueva, L., Levina, L., Hines, M. A., Cyr, P. W., & Sargent, E. H. (2004) · Applied Physics Letters · doi:10.1063/1.1755414 · Cited by 93
Analysis of a full spectrum hybrid lighting system
Schlegel, G., Burkholder, F., Klein, S. A., Beckman, W. A., Wood, B. D., & Muhs, J. D. (2003) · Solar Energy · doi:10.1016/j.solener.2003.11.005 · Cited by 69
High near-infrared photoluminescence quantum efficiency from PbS nanocrystals in polymer films
Chang, T.-W. F., Maria, A., Cyr, P. W., Sukhovatkin, V., Levina, L., & Sargent, E. H. (2004) · Synthetic Metals · doi:10.1016/j.synthmet.2004.10.003 · Cited by 44
Fruitfly centre spreads its wings
Dalton, R. (2000) · Nature · doi:10.1038/35044258 · Cited by 10
Cited by
Emergence of colloidal quantum-dot light-emitting technologies
Shirasaki, Y., Supran, G. J., Bawendi, M. G., & Bulović, V. (2013) · Nature Photonics · doi:10.1038/nphoton.2012.328 · Cited by 2,635
High-Detectivity Polymer Photodetectors with Spectral Response from 300 nm to 1450 nm
Gong, X., Tong, M., Xia, Y., Cai, W., Moon, J. S., Cao, Y., Yu, G., Shieh, C.-L., Nilsson, B., & Heeger, A. J. (2009) · Science · doi:10.1126/science.1176706 · Cited by 1,919
Ultrasensitive solution-cast quantum dot photodetectors
Konstantatos, G., Howard, I., Fischer, A., Hoogland, S., Clifford, J., Klem, E., Levina, L., & Sargent, E. H. (2006) · Nature · doi:10.1038/nature04855 · Cited by 1,883
Size-Dependent Optical Properties of Colloidal PbS Quantum Dots
Moreels, I., Lambert, K., Smeets, D., De Muynck, D., Nollet, T., Martins, J. C., Vanhaecke, F., Vantomme, A., Delerue, C., Allan, G., et al. (2009) · ACS Nano · doi:10.1021/nn900863a · Cited by 1,249
Nanoparticulate Functional Materials
Goesmann, H., & Feldmann, C. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.200903053 · Cited by 733
Metadata
- Authors
- H. Sargent, E.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2005-03-03
- Volume
- 17
- Issue
- 5
- Pages
- 515-522
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W1978278799
- Cited by
- 552
- References
- 23
- FWCI
- 19.35
- Type
- journal article
- Language
- en
- Open access
- closed
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