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Vertically Aligned Ta3N5 Nanorod Arrays for Solar‐Driven Photoelectrochemical Water Splitting
Abstract
A vertically aligned Ta(3)N(5) nanorod photoelectrode is fabricated by through-mask anodization and nitridation for water splitting. The Ta(3)N(5) nanorods, working as photoanodes of a photoelectrochemical cell, yield a high photocurrent density of 3.8 mA cm(-2) at 1.23 V versus a reversible hydrogen electrode under AM 1.5G simulated sunlight and an incident photon-to-current conversion efficiency of 41.3% at 440 nm, one of the highest activities reported for photoanodes so far.
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Citations
Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Cited by
Yang, W., Prabhakar, R. R., Tan, J., Tilley, S. D., & Moon, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00997j · Cited by 787
Li, X., Wen, J., Low, J., Fang, Y., & Yu, J. (2014) · Science China Materials · doi:10.1007/s40843-014-0003-1 · Cited by 517
Tantalum-based semiconductors for solar water splitting
Zhang, P., Zhang, J., & Gong, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60438a · Cited by 494
Photocatalytic and Photoelectrochemical Systems: Similarities and Differences
Wu, H., Tan, H. L., Toe, C. Y., Scott, J., Wang, L., Amal, R., & Ng, Y. H. (2020) · Advanced Materials · doi:10.1002/adma.201904717 · Cited by 394
Li, Y., Zhang, L., Torres-Pardo, A., González-Calbet, J. M., Ma, Y., Oleynikov, P., Terasaki, O., Asahina, S., Shima, M., Cha, D., et al. (2013) · Nature Communications · doi:10.1038/ncomms3566 · Cited by 347
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Metadata
- Authors
- Li, Y., Takata, T., Cha, D., Takanabe, K., Minegishi, T., Kubota, J., & Domen, K.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2012-09-18
- Volume
- 25
- Issue
- 1
- Pages
- 125-131
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2115116732
- Cited by
- 407
- References
- 2
- FWCI
- 14.46
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, Y., Takata, T., Cha, D., Takanabe, K., Minegishi, T., Kubota, J., & Domen, K. (2013). Vertically Aligned Ta3N5 Nanorod Arrays for Solar‐Driven Photoelectrochemical Water Splitting. Advanced Materials. https://doi.org/10.1002/adma.201202582
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