Directed Growth of Metal‐Organic Frameworks and Their Derived Carbon‐Based Network for Efficient Electrocatalytic Oxygen Reduction
Abstract
A honeycomb-like carbon-based network is obtained by in situ nucleation and directed growth of metal-organic framework (MOF) arrays on the surface of layered double hydroxide (LDH) nanoplatelets, followed by a subsequent pyrolysis process, which exhibits largely enhanced electrocatalytic ORR performances. A successful paradigm for the directed growth of highly oriented MOF arrays is demonstrated, with potential applications for energy storage and conversion.
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By deconvolution, two Co species can be identified: Co2+ (Co-Ny) at 780.5 eV and Co3+ (CoCxNy) at 782 eV.
“By deconvolution, two distinguished Co species can be identified, where Co2+ (Co-Ny) fitting peak centered at 780.5 eV, and Co3+ (CoCxNy) fitting peak centered at 782 eV (Fig. S5b) [55].”
Cites
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
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Shao, Y., Sui, J., Yin, G., & Gao, Y. (2008) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2007.09.047 · Cited by 763 · see citing works
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MOF-derived nanohybrids for electrocatalysis and energy storage: current status and perspectives
Zhang, H., Liu, X., Wu, Y., Guan, C., Cheetham, A. K., & Wang, J. (2018) · Chemical Communications · doi:10.1039/c8cc00789f · Cited by 309 · see citing works
Zou, H., Li, G., Duan, L., Kou, Z., & Wang, J. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.118100 · Cited by 159 · see citing works
Chakraborty, A., & Acharya, H. (2018) · Colloid and Interface Science Communications · doi:10.1016/j.colcom.2018.03.005 · Cited by 63 · see citing works
Wang, X., Fei, Y., Wang, W., Yuan, W., & Li, C. M. (2019) · ACS Applied Energy Materials · doi:10.1021/acsaem.9b01861 · Cited by 40 · see citing works
- Authors
- Li, Z., Shao, M., Zhou, L., Zhang, R., Zhang, C., Wei, M., Evans, D. G., & Duan, X.
- Affiliations
- State Key Laboratory of Chemical Resource Engineering (CN)
- Corresponding author
- Shao, Mingfei
- Wei, Min
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2016-01-25
- Volume
- 28
- Issue
- 12
- Pages
- 2337-2344
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2265829476
- Cited by
- 498
- References
- 2
- Citations by year
- 2026: 10 · 2025: 17 · 2024: 18 · 2023: 28 · 2022: 51 · 2021: 53 · 2020: 70 · 2019: 71 · 2018: 84 · 2017: 70 · 2016: 26
- FWCI
- 22.72
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Advanced Materials (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Natural Science Foundation of China
- 973 Program (2014CB932102)
- China National Funds for Distinguished Young Scientists of the NSFC
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Keywords
- metal-organic frameworks, oxygen reduction reaction, electrocatalysis, in situ nucleation, pyrolysis, carbon-based electrocatalysts
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