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Hybrid Perovskite Light‐Emitting Diodes Based on Perovskite Nanocrystals with Organic–Inorganic Mixed Cations

Zhang, Xiaoli, Liu, He, Wang, Weigao, Zhang, Jinbao, Xu, Bing, Karen, Ke Lin, Zheng, Yuanjin, Liu, Sheng, Chen, Shuming, Wang, Kai, Sun, Xiao Wei·2017·Advanced Materials

Abstract

Organic–inorganic hybrid perovskite materials with mixed cations have demonstrated tremendous advances in photovoltaics recently, by showing a significant enhancement of power conversion efficiency and improved perovskite stability. Inspired by this development, this study presents the facile synthesis of mixed‐cation perovskite nanocrystals based on FA(1−x)CsxPbBr 3 (FA = CH(NH 2)2). By detailed characterization of their morphological, optical, and physicochemical properties, it is found that the emission property of the perovskite, FA(1−x)CsxPbBr 3, is significantly dependent on the substitution content of the Cs cations in the perovskite composition. These mixed‐cation perovskites are employed as light emitters in light‐emitting diodes (LEDs). With an optimized composition of FA 0.8 Cs 0.2 PbBr 3, the LEDs exhibit encouraging performance with a highest reported luminance of 55 005 cd m−2 and a current efficiency of 10.09 cd A−1. This work provides important instructions on the future compositional optimization of mixed‐cation perovskite for obtaining high‐performance LEDs. The authors believe this work is a new milestone in the development of bright and efficient perovskite LEDs.

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Metadata

Authors
Zhang, X., Liu, H., Wang, W., Zhang, J., Xu, B., Karen, K. L., Zheng, Y., Liu, S., Chen, S., Wang, K., & Sun, X. W.
Venue
Advanced Materials
Publisher
Wiley
Published
2017-03-07
Volume
29
Issue
18
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
OpenAlex
W2594334693
Cited by
296
References
2
FWCI
17.68
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Hybrid Perovskite Light‐Emitting Diodes Based on Perovskite Nanocrystals with Organic–Inorganic Mixed Cations. https://app.cochat.ai/papers/10.1002/adma.201606405
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Zhang, X., Liu, H., Wang, W., Zhang, J., Xu, B., Karen, K. L., Zheng, Y., Liu, S., Chen, S., Wang, K., & Sun, X. W. (2017). Hybrid Perovskite Light‐Emitting Diodes Based on Perovskite Nanocrystals with Organic–Inorganic Mixed Cations. Advanced Materials. https://doi.org/10.1002/adma.201606405

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