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A Nonmetal Plasmonic Z‐Scheme Photocatalyst with UV‐ to NIR‐Driven Photocatalytic Protons Reduction
Abstract
Ultrabroad‐spectrum absorption and highly efficient generation of available charge carriers are two essential requirements for promising semiconductor‐based photocatalysts, towards achieving the ultimate goal of solar‐to‐fuel conversion. Here, a fascinating nonmetal plasmonic Z‐scheme photocatalyst with the W 18 O 49/g‐C 3 N 4 heterostructure is reported, which can effectively harvest photon energies spanning from the UV to the nearinfrared region and simultaneously possesses improved charge‐carrier dynamics to boost the generation of long‐lived active electrons for the photocatalytic reduction of protons into H 2. By combining with theoretical simulations, a unique synergistic photocatalysis effect between the semiconductive Z‐scheme charge‐carrier separation and metal‐like localized‐surface‐plasmon‐resonance‐induced “hot electrons” injection process is demonstrated within this binary heterostructure.
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Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Cited by
Cocatalysts for Selective Photoreduction of CO2into Solar Fuels
Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Direct Z-scheme photocatalysts: Principles, synthesis, and applications
Xu, Q., Zhang, L., Yu, J., Wageh, S., Al-Ghamdi, A. A., & Jaroniec, M. (2018) · Materials Today · doi:10.1016/j.mattod.2018.04.008 · Cited by 1,635
Zhu, M., Kim, S., Mao, L., Fujitsuka, M., Zhang, J., Wang, X., & Majima, T. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b08416 · Cited by 1,040
Photocatalysis: From Fundamental Principles to Materials and Applications
Yang, X., & Wang, D. (2018) · ACS Applied Energy Materials · doi:10.1021/acsaem.8b01345 · Cited by 770
Half-unit-cell ZnIn2S4 monolayer with sulfur vacancies for photocatalytic hydrogen evolution
Du, C., Zhang, Q., Lin, Z., Yan, B., Xia, C., & Yang, G. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.02.027 · Cited by 621
Metadata
- Authors
- Zhang, Z., Huang, J., Fang, Y., Zhang, M., Liu, K., & Dong, B.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-03-06
- Volume
- 29
- Issue
- 18
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2593743439
- Cited by
- 519
- References
- 2
- FWCI
- 16.51
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, Z., Huang, J., Fang, Y., Zhang, M., Liu, K., & Dong, B. (2017). A Nonmetal Plasmonic Z‐Scheme Photocatalyst with UV‐ to NIR‐Driven Photocatalytic Protons Reduction. Advanced Materials. https://doi.org/10.1002/adma.201606688
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