The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
In Situ Transformation of MOFs into Layered Double Hydroxide Embedded Metal Sulfides for Improved Electrocatalytic and Supercapacitive Performance
Abstract
Direct adoption of metal‐organic frameworks (MOFs) as electrode materials shows impoverished electrochemical performance owing to low electrical conductivity and poor chemical stability. In this study, we demonstrate self‐templated pseudomorphic transformation of MOF into surface chemistry rich hollow framework that delivers highly reactive, durable, and universal electrochemically active energy conversion and storage functionalities. In situ pseudomorphic transformation of MOF‐derived hollow rhombic dodecahedron template and sulfurization of nickel cobalt layered double hydroxides (NiCo‐LDHs) lead to the construction of interlayered metal sulfides (NiCo‐LDH/Co 9 S 8) system. The embedment of metal sulfide species (Co 9 S 8) at the LDH intergalleries offers optimal interfacing of the hybrid constituent elements and materials stability. The hybrid NiCo‐LDH/Co 9 S 8 system collectively presents an ideal porous structure, rich redox chemistry, and high electrical conductivity matrix. This leads to a significant enhancement in its complementary electrocatalytic hydrogen evolution and supercapacitive energy storage properties. This work establishes the potential of MOF derived scaffold for designing of novel class hybrid inorganic–organic functional materials for electrochemical applications and beyond.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Huang, Z.-F., Song, J., Li, K., Tahir, M., Wang, Y.-T., Pan, L., Wang, L., Zhang, X., & Zou, J.-J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.5b11986 · Cited by 749
Cited by
Nanoarchitectonics for Transition‐Metal‐Sulfide‐Based Electrocatalysts for Water Splitting
Guo, Y., Park, T., Yi, J. W., Henzie, J., Kim, J., Wang, Z., Jiang, B., Bando, Y., Sugahara, Y., Tang, J., et al. (2019) · Advanced Materials · doi:10.1002/adma.201807134 · Cited by 1,402
Su, J., Ge, R., Jiang, K., Dong, Y., Hao, F., Tian, Z., Chen, G., & Chen, L. (2018) · Advanced Materials · doi:10.1002/adma.201801351 · Cited by 544
Wang, C., Kaneti, Y. V., Bando, Y., Lin, J., Liu, C., Li, J., & Yamauchi, Y. (2018) · Materials Horizons · doi:10.1039/c8mh00133b · Cited by 533
Recent progress in metal-organic frameworks as active materials for supercapacitors
Wang, K.-B., Xun, Q., & Zhang, Q. (2020) · EnergyChem · doi:10.1016/j.enchem.2019.100025 · Cited by 474
Cheng, N., Ren, L., Xu, X., Du, Y., & Dou, S. X. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201801257 · Cited by 359
Metadata
- Authors
- Yilmaz, G., Yam, K. M., Zhang, C., Fan, H. J., & Ho, G. W.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-05-03
- Volume
- 29
- Issue
- 26
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2610171426
- Cited by
- 643
- References
- 2
- FWCI
- 21.47
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yilmaz, G., Yam, K. M., Zhang, C., Fan, H. J., & Ho, G. W. (2017). In Situ Transformation of MOFs into Layered Double Hydroxide Embedded Metal Sulfides for Improved Electrocatalytic and Supercapacitive Performance. Advanced Materials. https://doi.org/10.1002/adma.201606814
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