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Cited by 589

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Ultrafast Formation of Amorphous Bimetallic Hydroxide Films on 3D Conductive Sulfide Nanoarrays for Large‐Current‐Density Oxygen Evolution Electrocatalysis

Zou, Xu, Liu, Yipu, Li, Guo‐Dong, Wu, Yuanyuan, Liu, Da‐Peng, Li, Wang, Li, Hai‐Wen, Wang, Dejun, Zhang, Yu, Zou, Xiaoxin·2017·Advanced Materials

Abstract

Developing nonprecious oxygen evolution electrocatalysts that can work well at large current densities is of primary importance in a viable water‐splitting technology. Herein, a facile ultrafast (5 s) synthetic approach is reported that produces a novel, efficient, non‐noble metal oxygen‐evolution nano‐electrocatalyst that is composed of amorphous Ni–Fe bimetallic hydroxide film‐coated, nickel foam (NF)‐supported, Ni 3 S 2 nanosheet arrays. The composite nanomaterial (denoted as Ni‐Fe‐OH@Ni 3 S 2/NF) shows highly efficient electrocatalytic activity toward oxygen evolution reaction (OER) at large current densities, even in the order of 1000 mA cm−2. Ni‐Fe‐OH@Ni 3 S 2/NF also gives an excellent catalytic stability toward OER both in 1 m KOH solution and in 30 wt% KOH solution. Further experimental results indicate that the effective integration of high catalytic reactivity, high structural stability, and high electronic conductivity into a single material system makes Ni‐Fe‐OH@Ni 3 S 2/NF a remarkable catalytic ability for OER at large current densities.

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Metadata

Authors
Zou, X., Liu, Y., Li, G., Wu, Y., Liu, D., Li, W., Li, H., Wang, D., Zhang, Y., & Zou, X.
Venue
Advanced Materials
Publisher
Wiley
Published
2017-03-29
Volume
29
Issue
22
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
OpenAlex
W2600878234
Cited by
589
References
8
FWCI
17.51
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Ultrafast Formation of Amorphous Bimetallic Hydroxide Films on 3D Conductive Sulfide Nanoarrays for Large‐Current‐Density Oxygen Evolution Electrocatalysis. https://app.cochat.ai/papers/10.1002/adma.201700404
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Zou, X., Liu, Y., Li, G., Wu, Y., Liu, D., Li, W., Li, H., Wang, D., Zhang, Y., & Zou, X. (2017). Ultrafast Formation of Amorphous Bimetallic Hydroxide Films on 3D Conductive Sulfide Nanoarrays for Large‐Current‐Density Oxygen Evolution Electrocatalysis. Advanced Materials. https://doi.org/10.1002/adma.201700404

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