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Laser‐Induced Graphene in Controlled Atmospheres: From Superhydrophilic to Superhydrophobic Surfaces
Abstract
The modification of graphene‐based materials is an important topic in the field of materials research. This study aims to expand the range of properties for laser‐induced graphene (LIG), specifically to tune the hydrophobicity and hydrophilicity of the LIG surfaces. While LIG is normally prepared in the air, here, using selected gas atmospheres, a large change in the water contact angle on the as‐prepared LIG surfaces has been observed, from 0° (superhydrophilic) when using O 2 or air, to >150° (superhydrophobic) when using Ar or H 2. Characterization of the newly derived surfaces shows that the different wetting properties are due to the surface morphology and chemical composition of the LIG. Applications of the superhydrophobic LIG are shown in oil/water separation as well as anti‐icing surfaces, while the versatility of the controlled atmosphere chamber fabrication method is demonstrated through the improved microsupercapacitor performance generated from LIG films prepared in an O 2 atmosphere.
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Cites
Graphene: Status and Prospects
Geim, A. K. (2009) · Science · doi:10.1126/science.1158877 · Cited by 13,942
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Cited by
3D Graphene Materials: From Understanding to Design and Synthesis Control
Sun, Z., Fang, S., & Hu, Y. H. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00083 · Cited by 543
Bioinspired Designs of Superhydrophobic and Superhydrophilic Materials
Si, Y., Dong, Z., & Jiang, L. (2018) · ACS Central Science · doi:10.1021/acscentsci.8b00504 · Cited by 507
Duy, L. X., Peng, Z., Li, Y., Zhang, J., Ji, Y., & Tour, J. M. (2018) · Carbon · doi:10.1016/j.carbon.2017.10.036 · Cited by 503
Self-citationLaser‐Induced Graphene Strain Sensors Produced by Ultraviolet Irradiation of Polyimide
Carvalho, A. F., Fernandes, A. J. S., Leitão, C., Deuermeier, J., Marques, A. C., Martins, R., Fortunato, E., & Costa, F. M. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201805271 · Cited by 384
Laser-Induced Graphene Triboelectric Nanogenerators
Stanford, M. G., Li, J. T., Chyan, Y., Wang, Z., Wang, W., & Tour, J. M. (2019) · ACS Nano · doi:10.1021/acsnano.9b02596 · Cited by 316
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Metadata
- Authors
- Li, Y., Luong, D. X., Zhang, J., Tarkunde, Y. R., Kittrell, C., Sargunaraj, F., Ji, Y., Arnusch, C. J., & Tour, J. M.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-05-12
- Volume
- 29
- Issue
- 27
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2612998291
- Cited by
- 405
- References
- 2
- FWCI
- 12.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, Y., Luong, D. X., Zhang, J., Tarkunde, Y. R., Kittrell, C., Sargunaraj, F., Ji, Y., Arnusch, C. J., & Tour, J. M. (2017). Laser‐Induced Graphene in Controlled Atmospheres: From Superhydrophilic to Superhydrophobic Surfaces. Advanced Materials. https://doi.org/10.1002/adma.201700496
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