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Ultra‐High Pyridinic N‐Doped Porous Carbon Monolith Enabling High‐Capacity K‐Ion Battery Anodes for Both Half‐Cell and Full‐Cell Applications
Abstract
An ultrahigh pyridinic N‐content‐doped porous carbon monolith is reported, and the content of pyridinic N reaches up to 10.1% in overall material (53.4 ± 0.9% out of 18.9 ± 0.4% N content), being higher than most of previously reported N‐doping carbonaceous materials, which exhibit greatly improved electrochemical performance for potassium storage, especially in term of the high reversible capacity. Remarkably, the pyridinic N‐doped porous carbon monolith (PNCM) electrode exhibits high initial charge capacity of 487 mAh g−1 at a current density of 20 mA g−1, which is one of the highest reversible capacities among all carbonaceous anodes for K‐ion batteries. Moreover, the K‐ion full cell is successfully assembled, demonstrating a high practical energy density of 153.5 Wh kg−1. These results make PNCM promising for practical application in energy storage devices and encourage more investigations on a similar potassium storage system.
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Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
Cited by
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Yang, W., Zhou, J., Wang, S., Zhang, W., Wang, Z., Lv, F., Wang, K., Sun, Q., & Guo, S. (2019) · Energy & Environmental Science · doi:10.1039/c9ee00536f · Cited by 404
An Overview and Future Perspectives of Rechargeable Zinc Batteries
Shi, Y., Chen, Y., Shi, L., Wang, K., Wang, B., Li, L., Ma, Y., Li, Y., Sun, Z., Ali, W., et al. (2020) · Small · doi:10.1002/smll.202000730 · Cited by 389
Self-citationN/O Dual‐Doped Environment‐Friendly Hard Carbon as Advanced Anode for Potassium‐Ion Batteries
Cui, R. C., Xu, B., Dong, H. J., Yang, C. C., & Jiang, Q. (2020) · Advanced Science · doi:10.1002/advs.201902547 · Cited by 302
Metadata
- Authors
- Xie, Y., Chen, Y., Liu, L., Tao, P., Fan, M., Xu, N., Shen, X., & Yan, C.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-07-17
- Volume
- 29
- Issue
- 35
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2736230196
- Cited by
- 405
- References
- 1
- FWCI
- 22.71
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xie, Y., Chen, Y., Liu, L., Tao, P., Fan, M., Xu, N., Shen, X., & Yan, C. (2017). Ultra‐High Pyridinic N‐Doped Porous Carbon Monolith Enabling High‐Capacity K‐Ion Battery Anodes for Both Half‐Cell and Full‐Cell Applications. Advanced Materials. https://doi.org/10.1002/adma.201702268
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