The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Thermal Exfoliation of Layered Metal–Organic Frameworks into Ultrahydrophilic Graphene Stacks and Their Applications in Li–S Batteries
Open accessAbstract
2D nanocarbon‐based materials with controllable pore structures and hydrophilic surface show great potential in electrochemical energy storage systems including lithium sulfur (Li–S) batteries. This paper reports a thermal exfoliation of metal–organic framework crystals with intrinsic 2D structure into multilayer graphene stacks. This family of nanocarbon stacks is composed of well‐preserved 2D sheets with highly accessible interlayer macropores, narrowly distributed 7 Å micropores, and ever most polar pore walls. The surface polarity is quantified both by its ultrahigh water vapor uptake of 14.3 mmol g−1 at low relative pressure of P/P0 = 0.4 and ultrafast water wetting capability in less than 10.0 s. Based on the structural merits, this series hydrophilic multilayer graphene stack is showcased as suitable model cathode host for unveiling the challenging surface chemistry issue in Li–S batteries.
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Wu, H. B., Xia, B. Y., Yu, L., Yu, X.-Y., & Lou, X. W. (2015) · Nature Communications · doi:10.1038/ncomms7512 · Cited by 1,434
Cited by
Wang, M., Fan, L., Sun, X., Guan, B., Jiang, B., Wu, X., Tian, D., Sun, K., Qiu, Y., Yin, X., et al. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.0c01564 · Cited by 312
Emerging 2D materials beyond graphene for ultrashort pulse generation in fiber lasers
He, J., Tao, L., Zhang, H., Zhou, B., & Li, J. (2019) · Nanoscale · doi:10.1039/c8nr09368g · Cited by 282
Hou, C., Zou, L., Wang, Y., & Xu, Q. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202011347 · Cited by 281
Metadata
- Authors
- Hao, G., Tang, C., Zhang, E., Zhai, P., Yin, J., Zhu, W., Zhang, Q., & Kaskel, S.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-08-07
- Volume
- 29
- Issue
- 37
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2745280953
- Cited by
- 169
- References
- 1
- FWCI
- 10.40
- Type
- journal article
- Language
- en
- Open access
- green
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