The DOI matches its Crossref record; 44 of the 44 references it cites were found in a registry or an index.
Flexible, High‐Wettability and Fire‐Resistant Separators Based on Hydroxyapatite Nanowires for Advanced Lithium‐Ion Batteries
Abstract
Separators play a pivotal role in the electrochemical performance and safety of lithium‐ion batteries (LIBs). The commercial microporous polyolefin‐based separators often suffer from inferior electrolyte wettability, low thermal stability, and severe safety concerns. Herein, a novel kind of highly flexible and porous separator based on hydroxyapatite nanowires (HAP NWs) with excellent thermal stability, fire resistance, and superior electrolyte wettability is reported. A hierarchical cross‐linked network structure forms between HAP NWs and cellulose fibers (CFs) via hybridization, which endows the separator with high flexibility and robust mechanical strength. The high thermal stability of HAP NW networks enables the separator to preserve its structural integrity at temperatures as high as 700 °C, and the fire‐resistant property of HAP NWs ensures high safety of the battery. In particular, benefiting from its unique composition and highly porous structure, the as‐prepared HAP/CF separator exhibits near zero contact angle with the liquid electrolyte and high electrolyte uptake of 253%, indicating superior electrolyte wettability compared with the commercial polyolefin separator. The as‐prepared HAP/CF separator has unique advantages of superior electrolyte wettability, mechanical robustness, high thermal stability, and fire resistance, thus, is promising as a new kind of separator for advanced LIBs with enhanced performance and high safety.
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Citations
Cites
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Cited by
High-safety separators for lithium-ion batteries and sodium-ion batteries: advances and perspective
Zhang, L., Li, X., Yang, M., & Chen, W. (2021) · Energy Storage Materials · doi:10.1016/j.ensm.2021.06.033 · Cited by 587
Nanowires for Electrochemical Energy Storage
Zhou, G., Xu, L., Hu, G., Mai, L., & Cui, Y. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00326 · Cited by 439
Costa, C. M., Lee, Y.-H., Kim, J.-H., Lee, S.-Y., & Lanceros-Méndez, S. (2019) · Energy Storage Materials · doi:10.1016/j.ensm.2019.07.024 · Cited by 369
Safer Lithium‐Ion Batteries from the Separator Aspect: Development and Future Perspectives
Liu, Z., Jiang, Y., Hu, Q., Guo, S., Yu, L., Li, Q., Liu, Q., & Hu, X. (2021) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12129 · Cited by 253
Self-citationNguyen, M. H., Zbair, M., Dutournié, P., Gervasini, A., Vaulot, C., & Bennici, S. (2022) · Solar Energy Materials and Solar Cells · doi:10.1016/j.solmat.2022.111696 · Cited by 52
Metadata
- Authors
- Li, H., Wu, D., Wu, J., Dong, L., Zhu, Y., & Hu, X.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-10-16
- Volume
- 29
- Issue
- 44
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2767157095
- Cited by
- 401
- References
- 44
- FWCI
- 13.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, H., Wu, D., Wu, J., Dong, L., Zhu, Y., & Hu, X. (2017). Flexible, High‐Wettability and Fire‐Resistant Separators Based on Hydroxyapatite Nanowires for Advanced Lithium‐Ion Batteries. Advanced Materials. https://doi.org/10.1002/adma.201703548
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