The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Layered‐Double‐Hydroxide Nanosheets as Efficient Visible‐Light‐Driven Photocatalysts for Dinitrogen Fixation
Abstract
Semiconductor photocatalysis attracts widespread interest in water splitting, CO 2 reduction, and N 2 fixation. N 2 reduction to NH 3 is essential to the chemical industry and to the Earth's nitrogen cycle. Industrially, NH 3 is synthesized by the Haber–Bosch process under extreme conditions (400–500 °C, 200–250 bar), stimulating research into the development of sustainable technologies for NH 3 production. Herein, this study demonstrates that ultrathin layered‐double‐hydroxide (LDH) photocatalysts, in particular CuCr‐LDH nanosheets, possess remarkable photocatalytic activity for the photoreduction of N 2 to NH 3 in water at 25 °C under visible‐light irradiation. The excellent activity can be attributed to the severely distorted structure and compressive strain in the LDH nanosheets, which significantly enhances N 2 chemisorption and thereby promotes NH 3 formation.
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Wang, P., Chang, F., Gao, W., Guo, J., Wu, G., He, T., & Chen, P. (2017) · Nature Chemistry · doi:10.1038/nchem.2595 · Cited by 711
Cited by
A Review of Electrocatalytic Reduction of Dinitrogen to Ammonia under Ambient Conditions
Cui, X., Tang, C., & Zhang, Q. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201800369 · Cited by 1,314
Zhao, Y., Waterhouse, G. I. N., Chen, G., Xiong, X., Wu, L.-Z., Tung, C.-H., & Zhang, T. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00607e · Cited by 435
Self-citationYang, M., Gao, M., Hong, M., & Ho, G. W. (2018) · Advanced Materials · doi:10.1002/adma.201802894 · Cited by 389
Photocatalytic nitrogen fixation: the role of defects in photocatalysts
Cheng, M., Xiao, C., & Xie, Y. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta06435d · Cited by 319
Chen, L.-W., Hao, Y.-C., Guo, Y., Zhang, Q., Li, J., Gao, W.-Y., Ren, L., Su, X., Hu, L., Zhang, N., et al. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.0c13342 · Cited by 303
Metadata
- Authors
- Zhao, Y., Zhao, Y., Waterhouse, G. I. N., Zheng, L., Cao, X., Teng, F., Wu, L., Tung, C., O'Hare, D., & Zhang, T.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-09-28
- Volume
- 29
- Issue
- 42
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2759485485
- Cited by
- 706
- References
- 1
- FWCI
- 23.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, Y., Zhao, Y., Waterhouse, G. I. N., Zheng, L., Cao, X., Teng, F., Wu, L., Tung, C., O'Hare, D., & Zhang, T. (2017). Layered‐Double‐Hydroxide Nanosheets as Efficient Visible‐Light‐Driven Photocatalysts for Dinitrogen Fixation. Advanced Materials. https://doi.org/10.1002/adma.201703828
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