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Rechargeable Aqueous Zinc‐Ion Battery Based on Porous Framework Zinc Pyrovanadate Intercalation Cathode
Abstract
In this work, a microwave approach is developed to rapidly synthesize ultralong zinc pyrovanadate (Zn 3 V 2 O 7(OH)2·2H 2 O, ZVO) nanowires with a porous crystal framework. It is shown that our synthesis strategy can easily be extended to fabricate other metal pyrovanadate compounds. The zinc pyrovanadate nanowires show significantly improved electrochemical performance when used as intercalation cathode for aqueous zinc–ion battery. Specifically, the ZVO cathode delivers high capacities of 213 and 76 mA h g−1 at current densities of 50 and 3000 mA g−1, respectively. Furthermore, the Zn//ZVO cells show good cycling stability up to 300 cycles. The estimated energy density of this Zn cell is ≈214Wh kg−1, which is much higher than commercial lead–acid batteries. Significant insight into the Zn‐storage mechanism in the pyrovanadate cathodes is presented using multiple analytical methods. In addition, it is shown that our prototype device can power a 1.5 V temperature sensor for at least 24 h.
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Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
Where do batteries end and supercapacitors begin?
Simon, P., Gogotsi, Y., & Dunn, B. (2014) · Science · doi:10.1126/science.1249625 · Cited by 5,634
Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
Zhang, N., Dong, Y., Jia, M., Bian, X., Wang, Y., Qiu, M., Xu, J., Liu, Y., Jiao, L., & Cheng, F. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b00565 · Cited by 1,052
Highly Durable Na2V6O16·1.63H2O Nanowire Cathode for Aqueous Zinc-Ion Battery
Hu, P., Zhu, T., Wang, X., Wei, X., Yan, M., Li, J., Luo, W., Yang, W., Zhang, W., Zhou, L., et al. (2018) · Nano Letters · doi:10.1021/acs.nanolett.7b04889 · Cited by 710
Yang, Q., Liang, G., Guo, Y., Liu, Z., Yan, B., Wang, D., Huang, Z., Li, X., Fan, J., & Zhi, C. (2019) · Advanced Materials · doi:10.1002/adma.201903778 · Cited by 689
Zeng, Y., Lai, Z., Han, Y., Zhang, H., Xie, S., & Lu, X. (2018) · Advanced Materials · doi:10.1002/adma.201802396 · Cited by 678
Metadata
- Authors
- Xia, C., Guo, J., Lei, Y., Liang, H., Zhao, C., & Alshareef, H. N.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-12-11
- Volume
- 30
- Issue
- 5
- Pages
- e1907798-e1907798
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2774004638
- Cited by
- 967
- References
- 2
- FWCI
- 36.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xia, C., Guo, J., Lei, Y., Liang, H., Zhao, C., & Alshareef, H. N. (2018). Rechargeable Aqueous Zinc‐Ion Battery Based on Porous Framework Zinc Pyrovanadate Intercalation Cathode. Advanced Materials. https://doi.org/10.1002/adma.201705580
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