The DOI matches its Crossref record; 11 of the 11 references it cites were found in a registry or an index.
Rhenium‐Doped and Stabilized MoS2 Atomic Layers with Basal‐Plane Catalytic Activity
Open accessAbstract
The development of stable and efficient hydrogen evolution reaction (HER) catalysts is essential for the production of hydrogen as a clean energy resource. A combination of experiment and theory demonstrates that the normally inert basal planes of 2D layers of MoS 2 can be made highly catalytically active for the HER when alloyed with rhenium (Re). The presence of Re at the ≈50% level converts the material to a stable distorted tetragonal (DT) structure that shows enhanced HER activity as compared to most of the MoS 2‐based catalysts reported in the literature. More importantly, this new alloy catalyst shows much better stability over time and cycling than lithiated 1T‐MoS 2. Density functional theory calculations find that the role of Re is only to stabilize the DT structure, while catalysis occurs primarily in local Mo‐rich DT configurations, where the HER catalytic activity is very close to that in Pt. The study provides a new strategy to improve the overall HER performance of MoS 2‐based materials via chemical doping.
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Confinement Catalysis with 2D Materials for Energy Conversion
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Roadmap and Direction toward High-Performance MoS 2 Hydrogen Evolution Catalysts
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2D Metallic Transition‐Metal Dichalcogenides: Structures, Synthesis, Properties, and Applications
Zhao, B., Shen, D., Zhang, Z., Lu, P., Hossain, M., Li, J., Li, B., & Duan, X. (2021) · Advanced Functional Materials · doi:10.1002/adfm.202105132 · Cited by 359
Metadata
- Authors
- Yang, S., Gong, Y., Manchanda, P., Zhang, Y., Ye, G., Chen, S., Song, L., Pantelides, S. T., Ajayan, P. M., Chisholm, M. F., & Zhou, W.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-10-25
- Volume
- 30
- Issue
- 51
- Pages
- e1803477-e1803477
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2898251294
- Cited by
- 234
- References
- 11
- FWCI
- 6.28
- Type
- journal article
- Language
- en
- Open access
- green
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- Yang, S., Gong, Y., Manchanda, P., Zhang, Y., Ye, G., Chen, S., Song, L., Pantelides, S. T., Ajayan, P. M., Chisholm, M. F., & Zhou, W. (2018). Rhenium‐Doped and Stabilized MoS2 Atomic Layers with Basal‐Plane Catalytic Activity. Advanced Materials. https://doi.org/10.1002/adma.201803477
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