The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Achieving a Record‐High Yield Rate of 120.9 for N2 Electrochemical Reduction over Ru Single‐Atom Catalysts
Abstract
The electrochemical reduction of N 2 into NH 3 production under ambient conditions represents an attractive prospect for the fixation of N 2. However, this process suffers from low yield rate of NH 3 over reported electrocatalysts. In this work, a record‐high activity for N 2 electrochemical reduction over Ru single atoms distributed on nitrogen‐doped carbon (Ru SAs/N‐C) is reported. At −0.2 V versus reversible hydrogen electrode, Ru SAs/N‐C achieves a Faradaic efficiency of 29.6% for NH 3 production with partial current density of −0.13 mA cm−2. Notably, the yield rate of Ru SAs/N‐C reaches 120.9 , which is one order of magnitude higher than the highest value ever reported. This work not only develops a superior electrocatalyst for NH 3 production, but also provides a guideline for the rational design of highly active and robust single‐atom catalysts.
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Montoya, J. H., Tsai, C., Vojvodic, A., & Nørskov, J. K. (2015) · ChemSusChem · doi:10.1002/cssc.201500322 · Cited by 1,384
Zhang, C., Sha, J., Fei, H., Liu, M., Yazdi, S., Zhang, J., Zhong, Q., Zou, X., Zhao, N., Yu, H., et al. (2017) · ACS Nano · doi:10.1021/acsnano.7b02148 · Cited by 545
Energy efficiency improvements in ammonia production—perspectives and uncertainties
Rafiqul, I., Weber, C., Lehmann, B., & Voss, A. (2005) · Energy · doi:10.1016/j.energy.2004.12.004 · Cited by 439
Cited by
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Liu, Y., Li, X., Zhang, Q., Li, W., Xie, Y., Liu, H., Shang, L., Liu, Z., Chen, Z., Gu, L., et al. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201913910 · Cited by 647
Self-citationFang, S., Zhu, X., Liu, X., Gu, J., Liu, W., Wang, D., Zhang, W., Lin, Y., Lu, J., Wei, S., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-14848-2 · Cited by 585
Defect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Lu, X. F., Fang, Y., Luan, D., & Lou, X. W. D. (2021) · Nano Letters · doi:10.1021/acs.nanolett.0c04898 · Cited by 555
Metadata
- Authors
- Geng, Z., Liu, Y., Kong, X., Li, P., Li, K., Liu, Z., Du, J., Shu, M., Si, R., & Zeng, J.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-08-10
- Volume
- 30
- Issue
- 40
- Pages
- e1803498-e1803498
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2887542968
- Cited by
- 913
- References
- 3
- FWCI
- 29.55
- Type
- journal article
- Language
- en
- Open access
- closed
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- Geng, Z., Liu, Y., Kong, X., Li, P., Li, K., Liu, Z., Du, J., Shu, M., Si, R., & Zeng, J. (2018). Achieving a Record‐High Yield Rate of 120.9 for N2 Electrochemical Reduction over Ru Single‐Atom Catalysts. Advanced Materials. https://doi.org/10.1002/adma.201803498
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