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Controlling Monomer Feeding Rate to Achieve Highly Crystalline Covalent Triazine Frameworks
Abstract
The synthesis of highly crystalline covalent triazine frameworks (CTFs) with ultrastrong covalent bonds (aromatic CN) from the triazine linkage presents a great challenge to synthetic chemists. Herein, the synthesis of highly crystalline CTFs via directly controlling the monomer feeding rate is reported. By tuning the feeding rate of monomers, the crystallization process can be readily governed in a controlled manner in an open system. The sample of CTF‐HUST‐HC1 with abundant exposed {001} crystal facets has the better crystallinity and thus is selected to study the effect of high crystallinity on photoelectric properties. Owing to the better separation of photogenerated electron–hole pairs and charge transfer, the obtained highly ordered CTF‐HUST‐HC1 has superior performance in the photocatalytic removal of nitric oxide (NO) than its lesser crystalline counterparts and g‐C 3 N 4.
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Citations
Cited by
New synthetic strategies toward covalent organic frameworks
Li, Y., Chen, W., Xing, G., Jiang, D., & Chen, L. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00199f · Cited by 658
Porous organic polymers: a promising platform for efficient photocatalysis
Zhang, T., Xing, G., Chen, W., & Chen, L. (2020) · Materials Chemistry Frontiers · doi:10.1039/c9qm00633h · Cited by 420
(2021) · doi:10.1038/s41467-021-26817-4 · Cited by 222
Machine Learning‐Assisted Design of Nitrogen‐Rich Covalent Triazine Frameworks Photocatalysts
Wu, M., Song, Z., Cui, Y., Fu, Z., Hong, K., Li, Q., Lyu, Z., Liu, W., & Wang, J. (2025) · Advanced Functional Materials · doi:10.1002/adfm.202413453 · Cited by 17
Wu, M., Sun, J., Cui, Y., Fan, L., Hong, K., Liu, W., Li, Q., Lyu, Z., & Wang, J. (2025) · Advanced Functional Materials · doi:10.1002/adfm.202505234 · Cited by 11
Metadata
- Authors
- Liu, M., Jiang, K., Ding, X., Wang, S., Zhang, C., Liu, J., Zhan, Z., Cheng, G., Li, B., Chen, H., Jin, S., & Tan, B.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-03-28
- Volume
- 31
- Issue
- 19
- Pages
- e1807865-e1807865
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2930815130
- Cited by
- 237
- References
- 0
- FWCI
- 11.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, M., Jiang, K., Ding, X., Wang, S., Zhang, C., Liu, J., Zhan, Z., Cheng, G., Li, B., Chen, H., Jin, S., & Tan, B. (2019). Controlling Monomer Feeding Rate to Achieve Highly Crystalline Covalent Triazine Frameworks. Advanced Materials. https://doi.org/10.1002/adma.201807865
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