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2D Metal–Organic Frameworks as Multifunctional Materials in Heterogeneous Catalysis and Electro/Photocatalysis
Abstract
Metal–organic frameworks (MOFs) are composed of particles with 3D geometry and are currently among the most widely studied heterogeneous catalysts. To further increase their activity, one of the recent trends is to develop related 2D materials with a high aspect ratio derived from a large lateral size and a small thickness. Here, the use of these 2D MOFs as catalysts, electrocatalysts, and photocatalysts is summarized, illustrating the advantages of these 2D materials compared to analogous 3D MOFs. The state of the art is summarized in tables and, when possible, pertinent turnover number (TON) and frequency (TOF) values. This enhanced activity of 2D MOFs derives from the accessibility of the active sites, the presence of a higher density of defects, and exchangeable coordination positions around the MOFs, as well as from their ability to form thin films on electrodes or surfaces. The importance of providing convincing evidence of the stability of 2D MOFs under reaction conditions and general characterization data of the used 2D material after catalysis is highlighted. In the last part, views regarding challenges in the field and new developments that can be expected are presented.
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Cites
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Metal-organic framework materials as catalysts
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Graphene–MoS2 hybrid structures for multifunctional photoresponsive memory devices
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Cited by
Huang, H., Zhao, Y., Bai, Y., Li, F., Zhang, Y., & Chen, Y. (2020) · Advanced Science · doi:10.1002/advs.202000012 · Cited by 335
Wu, Y., Li, Y., Gao, J., & Zhang, Q. (2021) · SusMat · doi:10.1002/sus2.3 · Cited by 319
Theoretical Advances in Understanding and Designing the Active Sites for Hydrogen Evolution Reaction
Sun, F., Tang, Q., & Jiang, D.-E. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c02081 · Cited by 285
Dislocated Bilayer MOF Enables High‐Selectivity Photocatalytic Reduction of CO2 to CO
Liang, J., Yu, H., Shi, J., Li, B., Wu, L., & Wang, M. (2023) · Advanced Materials · doi:10.1002/adma.202209814 · Cited by 270
Yan, Y., Li, C., Wu, Y., Gao, J., & Zhang, Q. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta03749d · Cited by 260
Metadata
- Authors
- Dhakshinamoorthy, A., Asiri, A. M., & Garcia, H.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-08-20
- Volume
- 31
- Issue
- 41
- Pages
- e1900617-e1900617
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2969531510
- Cited by
- 462
- References
- 5
- FWCI
- 21.89
- Type
- journal article
- Language
- en
- Open access
- closed
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