The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Supported Noble‐Metal Single Atoms for Heterogeneous Catalysis
Abstract
Single‐atom catalysts (SACs), with atomically distributed active metal sites on supports, serve as a newly advanced material in catalysis, and open broad prospects for a wide variety of catalytic processes owing to their unique catalytic behaviors. To construct SACs with precise structures and high density of accessible single‐atom sites, while preventing aggregation to large nanoparticles, various strategies for their chemical synthesis have been recently developed by improving the distribution and chemical bonding of active sites on supports, which results in excellent activity and selectivity in a variety of catalytic reactions. Noble‐metal‐based SACs are discussed, and their structural properties, chemical synthesis, and catalytic applications are highlighted. The structure–activity relationships and the underlying catalytic mechanisms are addressed, including the influences of surface species and reducibility of supports on the activity and stability, impact of the unique structural and electronic properties of single‐atom centers modulated by metal/support interactions on catalytic activity and selectivity, and how the modified catalytic mechanism obtained by inhibiting the multiatoms involves catalytic pathways. Finally, the prospects and challenges for development in this field are highlighted.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Self-citationMontoya, J. H., Tsai, C., Vojvodic, A., & Nørskov, J. K. (2015) · ChemSusChem · doi:10.1002/cssc.201500322 · Cited by 1,384
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Back, S., Lim, J., Kim, N.-Y., Kim, Y.-H., & Jung, Y. (2017) · Chemical Science · doi:10.1039/c6sc03911a · Cited by 542
Cited by
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
Jiao, L., Yang, W., Wan, G., Zhang, R., Zheng, X., Zhou, H., Yu, S., & Jiang, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202008787 · Cited by 412
Wang, Y., Liu, Y., Liu, W., Wu, J., Li, Q., Feng, Q., Chen, Z., Xiong, X., Wang, D., & Lei, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02833a · Cited by 303
Improving the HER Activity and Stability of Pt Nanoparticles by Titanium Oxynitride Support
Smiljanić, M., Panić, S., Bele, M., Ruiz-Zepeda, F., Pavko, L., Gašparič, L., Kokalj, A., Gaberšček, M., & Hodnik, N. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c03214 · Cited by 203
Yang, Z., Chen, C., Zhao, Y., Wang, Q., Zhao, J., Waterhouse, G. I. N., Qin, Y., Shang, L., & Zhang, T. (2023) · Advanced Materials · doi:10.1002/adma.202208799 · Cited by 120
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Metadata
- Authors
- Li, X., Yang, X., Huang, Y., Zhang, T., & Liu, B.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-07-07
- Volume
- 31
- Issue
- 50
- Pages
- e1902031-e1902031
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2960957244
- Cited by
- 372
- References
- 5
- FWCI
- 14.76
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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