The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
A Highly Crystalline Perylene Imide Polymer with the Robust Built‐In Electric Field for Efficient Photocatalytic Water Oxidation
Abstract
A highly crystalline perylene imide polymer (Urea‐PDI) photocatalyst is successfully constructed. The Urea‐PDI presents a wide spectrum response owing to its large conjugated system. The Urea‐PDI performs so far highest oxygen evolution rate (3223.9 µmol g−1 h−1) without cocatalysts under visible light. The performance is over 107.5 times higher than that of the conventional PDI supramolecular photocatalysts. The strong oxidizing ability comes from the deep valence band (+1.52 eV) which is contributed by the covalent‐bonded conjugated molecules. Besides, the high crystallinity and the large molecular dipoles of the Urea‐PDI contribute to a robust built‐in electric field promoting the separation and transportation of photogenerated carriers. Moreover, the Urea‐PDI is very stable and has no performance attenuation after 100 h continuous irradiation. The Urea‐PDI polymer photocatalyst provides with a new platform for the use of photocatalytic water oxidation, which is expected to contribute to clean energy production.
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Cites
Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
Cited by
Zhao, D., Wang, Y., Dong, C.-L., Huang, Y.-C., Chen, J., Xue, F., Shen, S., & Guo, L. (2021) · Nature Energy · doi:10.1038/s41560-021-00795-9 · Cited by 1,379
Jing, J., Yang, J., Li, W., Wu, Z., & Zhu, Y. (2022) · Advanced Materials · doi:10.1002/adma.202106807 · Cited by 367
Self-citationLi, X., Wang, W., Dong, F., Zhang, Z., Han, L., Luo, X., Huang, J., Feng, Z., Chen, Z., Jia, G., et al. (2021) · ACS Catalysis · doi:10.1021/acscatal.0c05354 · Cited by 357
Self-citationYang, J., Jing, J., & Zhu, Y. (2021) · Advanced Materials · doi:10.1002/adma.202101026 · Cited by 293
Self-citationGuo, Y., Zhou, Q., Nan, J., Shi, W., Cui, F., & Zhu, Y. (2022) · Nature Communications · doi:10.1038/s41467-022-29826-z · Cited by 284
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Metadata
- Authors
- Zhang, Z., Chen, X., Zhang, H., Liu, W., Zhu, W., & Zhu, Y.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-06-28
- Volume
- 32
- Issue
- 32
- Pages
- e1907746-e1907746
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3037157774
- Cited by
- 364
- References
- 1
- FWCI
- 9.01
- Type
- journal article
- Language
- en
- Open access
- closed
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