The DOI matches its Crossref record; 9 of the 9 references it cites were found in a registry or an index.
Stable Rhodium (IV) Oxide for Alkaline Hydrogen Evolution Reaction
Abstract
Water electrolysis in alkaline electrolyte is an attractive way toward clean hydrogen energy via the hydrogen evolution reaction (HER), whereas the sluggish water dissociation impedes the following hydrogen evolution. Noble metal oxides possess promising capability for catalyzing water dissociation and hydrogen evolution; however, they are never utilized for the HER due to the instability under the reductive potential. Here it is shown that compressive strain can stabilize RhO 2 clusters and promote their catalytic activity. To this end, a strawberry‐like structure with RhO 2 clusters embedded in the surface layer of Rh nanoparticles is engineered, in which the incompatibility between the oxide cluster and the metal substrate causes intensive compressive strain. As such, RhO 2 clusters remain stable at a reduction potential up to −0.3 V versus reversible hydrogen electrode and present an alkaline HER activity superior to commercial Pt/C.
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Cites
Noble metal-free hydrogen evolution catalysts for water splitting
Zou, X., & Zhang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00448e · Cited by 5,955
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Nanostructured hydrotreating catalysts for electrochemical hydrogen evolution
Morales-Guio, C. G., Stern, L.-A., & Hu, X. (2014) · Chemical Society Reviews · doi:10.1039/c3cs60468c · Cited by 2,437
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
Liu, D., Li, X., Chen, S., Yan, H., Wang, C., Wu, C., Haleem, Y. A., Duan, S., Lu, J., Ge, B., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0402-6 · Cited by 1,166
High Electrocatalytic Hydrogen Evolution Activity of an Anomalous Ruthenium Catalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Jaroniec, M., & Qiao, S.-Z. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b11291 · Cited by 1,110
Activating cobalt(II) oxide nanorods for efficient electrocatalysis by strain engineering
Ling, T., Yan, D.-Y., Wang, H., Jiao, Y., Hu, Z., Zheng, Y., Zheng, L., Mao, J., Liu, H., Du, X.-W., et al. (2017) · Nature Communications · doi:10.1038/s41467-017-01872-y · Cited by 450
Self-citationUltrahigh-current-density niobium disulfide catalysts for hydrogen evolution
Yang, J., Mohmad, A. R., Wang, Y., Fullon, R., Song, X., Zhao, F., Bozkurt, I., Augustin, M., Santos, E. J. G., Shin, H. S., et al. (2019) · Nature Materials · doi:10.1038/s41563-019-0463-8 · Cited by 401
Jiang, R., Tran, D. T., Li, J., & Chu, D. (2019) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12031 · Cited by 112
Cited by
Tan, H., Tang, B., Lu, Y., Ji, Q., Lv, L., Duan, H., Li, N., Wang, Y., Feng, S., Li, Z., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-29710-w · Cited by 390
Self-citationLiu, Y., Wang, Q., Zhang, J., Ding, J., Cheng, Y., Wang, T., Li, J., Hu, F., Yang, H. B., & Liu, B. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202200928 · Cited by 304
Liu, Y., Ding, J., Li, F., Su, X., Zhang, Q., Guan, G., Hu, F., Zhang, J., Wang, Q., Jiang, Y., et al. (2023) · Advanced Materials · doi:10.1002/adma.202207114 · Cited by 193
Atomically Dispersed MoO x on Rhodium Metallene Boosts Electrocatalyzed Alkaline Hydrogen Evolution
Wu, J., Fan, J., Zhao, X., Wang, Y., Wang, D., Liu, H., Gu, L., Zhang, Q., Zheng, L., Singh, D. J., et al. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202207512 · Cited by 123
Self-citationRecent progress and perspective of electrocatalysts for the hydrogen evolution reaction
Shi, J., Bao, Y., Ye, R., Zhong, J., Zhou, L., Zhao, Z., Kang, W., & Aidarova, S. B. (2025) · Catalysis Science & Technology · doi:10.1039/d4cy01449a · Cited by 106
Metadata
- Authors
- Li, Z., Feng, Y., Liang, Y., Cheng, C., Dong, C., Liu, H., & Du, X.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-05-17
- Volume
- 32
- Issue
- 25
- Pages
- e1908521-e1908521
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3024419935
- Cited by
- 170
- References
- 9
- FWCI
- 6.02
- Type
- journal article
- Language
- en
- Open access
- closed
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