The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
A Stimulus‐Responsive Zinc–Iodine Battery with Smart Overcharge Self‐Protection Function
Open accessAbstract
Zinc–iodine aqueous batteries (ZIABs) are highly attractive for grid‐scale energy storage due to their high theoretical capacities, environmental friendliness, and intrinsic non‐flammability. However, because of the close redox potential of Zn stripping/platting and hydrogen evolution, slight overcharge of ZIABs would induce drastic side reactions, serious safety concerns, and battery failure. A novel type of stimulus‐responsive zinc–iodine aqueous battery (SR‐ZIAB) with fast overcharge self‐protection ability is demonstrated by employing a smart pH‐responsive electrolyte. Operando spectroelectrochemical characterizations reveal that the battery failure mechanism of ZIABs during overcharge arises from the increase of electrolyte pH induced by hydrogen evolution as well as the consequent irreversible formation of insulating ZnO at anode and soluble Zn(IO 3)2 at cathode. Under overcharge conditions, the designed SR‐ZIABs can be rapidly switched off with capacity degrading to 6% of the initial capacity, thereby avoiding continuous battery damage. Importantly, SR‐ZIABs can be switched on with nearly 100% of capacity recovery by re‐adjusting the electrolyte pH. This work will inspire the development of aqueous Zn batteries with smart self‐protection ability in the overcharge state.
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Cites
3D Printed Photoresponsive Devices Based on Shape Memory Composites
Yang, H., Leow, W. R., Wang, T., Wang, J., Yu, J., He, K., Qi, D., Wan, C., & Chen, X. (2017) · Advanced Materials · doi:10.1002/adma.201701627 · Cited by 483
Cited by
Recent Advances of Aqueous Rechargeable Zinc‐Iodine Batteries: Challenges, Solutions, and Prospects
Lin, D., & Li, Y. (2022) · Advanced Materials · doi:10.1002/adma.202108856 · Cited by 470
Yu, M., Chandrasekhar, N., Raghupathy, R. K. M., Ly, K. H., Zhang, H., Dmitrieva, E., Liang, C., Lu, X., Kühne, T. D., Mirhosseini, H., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c07992 · Cited by 406
Self-citationHistorical development and novel concepts on electrolytes for aqueous rechargeable batteries
Chen, S., Zhang, M., Zou, P., Sun, B., & Tao, S. (2022) · Energy & Environmental Science · doi:10.1039/d2ee00004k · Cited by 308
Metadata
- Authors
- Wang, F., Tseng, J., Liu, Z., Zhang, P., Wang, G., Chen, G., Wu, W., Yu, M., Wu, Y., & Feng, X.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-03-05
- Volume
- 32
- Issue
- 16
- Pages
- e2000287-e2000287
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3009205659
- Cited by
- 174
- References
- 1
- FWCI
- 8.95
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Wang, F., Tseng, J., Liu, Z., Zhang, P., Wang, G., Chen, G., Wu, W., Yu, M., Wu, Y., & Feng, X. (2020). A Stimulus‐Responsive Zinc–Iodine Battery with Smart Overcharge Self‐Protection Function. Advanced Materials. https://doi.org/10.1002/adma.202000287
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