The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
A Tensile‐Strained Pt–Rh Single‐Atom Alloy Remarkably Boosts Ethanol Oxidation
Abstract
The rational design and control of electrocatalysts at single‐atomic sites could enable unprecedented atomic utilization and catalytic properties, yet it remains challenging in multimetallic alloys. Herein, the first example of isolated Rh atoms on ordered PtBi nanoplates (PtBi‐Rh 1) by atomic galvanic replacement, and their subsequent transformation into a tensile‐strained Pt–Rh single‐atom alloy (PtBi@PtRh 1) via electrochemical dealloying are presented. Benefiting from the Rh 1‐tailored Pt (110) surface with tensile strain, the PtBi@PtRh 1 nanoplates exhibit record‐high and all‐round superior electrocatalytic performance including activity, selectivity, stability, and anti‐poisoning ability toward ethanol oxidation in alkaline electrolytes. Density functional theory calculations reveal the synergism between effective Rh 1 and tensile strain in boosting the adsorption of ethanol and key surface intermediates and the CC bond cleavage of the intermediates. The facile synthesis of the tensile‐strained single‐atom alloy provides a novel strategy to construct model nanostructures, accelerating the development of highly efficient electrocatalysts.
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Cites
Liu, D., Li, X., Chen, S., Yan, H., Wang, C., Wu, C., Haleem, Y. A., Duan, S., Lu, J., Ge, B., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0402-6 · Cited by 1,166
Strain-controlled electrocatalysis on multimetallic nanomaterials
Luo, M., & Guo, S. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.59 · Cited by 1,115
Single-atom Rh/N-doped carbon electrocatalyst for formic acid oxidation
Xiong, Y., Dong, J., Huang, Z.-Q., Xin, P., Chen, W., Wang, Y., Li, Z., Jin, Z., Xing, W., Zhuang, Z., et al. (2020) · Nature Nanotechnology · doi:10.1038/s41565-020-0665-x · Cited by 610
Self-citationDu, R., Wang, J., Wang, Y., Hübner, R., Fan, X., Senkovska, I., Hu, Y., Kaskel, S., & Eychmüller, A. (2020) · Nature Communications · doi:10.1038/s41467-020-15391-w · Cited by 184
Cited by
Zhu, Y., Klingenhof, M., Gao, C., Koketsu, T., Weiser, G., Pi, Y., Liu, S., Sui, L., Hou, J., Li, J., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-45654-9 · Cited by 444
Toward Electrocatalytic Methanol Oxidation Reaction: Longstanding Debates and Emerging Catalysts
Wang, J., Zhang, B., Guo, W., Wang, L., Chen, J., Pan, H., & Sun, W. (2023) · Advanced Materials · doi:10.1002/adma.202211099 · Cited by 339
Challenges and Opportunities in Engineering the Electronic Structure of Single-Atom Catalysts
Giulimondi, V., Mitchell, S., & Pérez-Ramírez, J. (2023) · ACS Catalysis · doi:10.1021/acscatal.2c05992 · Cited by 292
Fan, X., Chen, W., Xie, L., Liu, X., Ding, Y., Zhang, L., Tang, M., Liao, Y., Yang, Q., Fu, X., et al. (2024) · Advanced Materials · doi:10.1002/adma.202313179 · Cited by 89
Self-citationZhang, R., Zhao, Y., Guo, Z., Liu, X., Zhu, L., & Jiang, Y. (2023) · Small · doi:10.1002/smll.202205587 · Cited by 24
Metadata
- Authors
- Luo, S., Zhang, L., Liao, Y., Li, L., Yang, Q., Wu, X., Wu, X., He, D., He, C., Chen, W., Wu, Q., Li, M., Hensen, E. J. M., & Quan, Z.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2021-03-22
- Volume
- 33
- Issue
- 17
- Pages
- e2008508-e2008508
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3138833923
- Cited by
- 199
- References
- 4
- FWCI
- 6.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Luo, S., Zhang, L., Liao, Y., Li, L., Yang, Q., Wu, X., Wu, X., He, D., He, C., Chen, W., Wu, Q., Li, M., Hensen, E. J. M., & Quan, Z. (2021). A Tensile‐Strained Pt–Rh Single‐Atom Alloy Remarkably Boosts Ethanol Oxidation. Advanced Materials. https://doi.org/10.1002/adma.202008508
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