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Ligand Modulation of Active Sites to Promote Electrocatalytic Oxygen Evolution
Abstract
Rationally designed catalysts hold the key to address the sluggish kinetics of oxygen evolution reaction (OER). However, engineering the active sites of such catalysts still faces grand challenges. This study proposes a feasible ligand modulation strategy to boost the OER catalytic activity of cobalt‐iron oxyhydroxide ((Fe,Co)OOH). The 2‐methylimidazole (MI) ligand coordination on (Fe,Co)OOH reduces the orbital overlap between the Fe/Co 3d and O 2p, which weakens the adsorption to oxygen‐containing intermediates and thus facilitates the unfavorable O 2 desorption. As a result, the MI ligand modulated (Fe,Co)OOH achieves an excellent OER performance with low overpotentials (230/290 mV at 10/100 mA cm‐2) and excellent durability (>155 h). This study provides a novel ligand modulation strategy for the design of OER catalysts.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Cited by
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Zhou, Y., Lu, R., Tao, X., Qiu, Z., Chen, G., Yang, J., Zhao, Y., Feng, X., & Müllen, K. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.2c12933 · Cited by 567
Self-citationMicroenvironment Engineering of Single/Dual‐Atom Catalysts for Electrocatalytic Application
Gao, Y., Liu, B., & Wang, D. (2023) · Advanced Materials · doi:10.1002/adma.202209654 · Cited by 319
Liu, H., Zhang, S., Chai, Y., & Dong, B. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202313845 · Cited by 188
Multicomponent transition metal oxides and (oxy)hydroxides for oxygen evolution
Han, J., & Guan, J. (2023) · Nano Research · doi:10.1007/s12274-022-4874-7 · Cited by 145
Li, Y., Yuan, M., Yang, H., Shi, K., Sun, Z., Li, H., Nan, C., & Sun, G. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2022.122167 · Cited by 55
Metadata
- Authors
- Huang, W., Li, J., Liao, X., Lu, R., Ling, C., Liu, X., Meng, J., Qu, L., Lin, M., Hong, X., Zhou, X., Liu, S., Zhao, Y., Zhou, L., & Mai, L.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2022-04-04
- Volume
- 34
- Issue
- 18
- Pages
- e2200270-e2200270
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W4221093064
- Cited by
- 254
- References
- 1
- FWCI
- 10.21
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, W., Li, J., Liao, X., Lu, R., Ling, C., Liu, X., Meng, J., Qu, L., Lin, M., Hong, X., Zhou, X., Liu, S., Zhao, Y., Zhou, L., & Mai, L. (2022). Ligand Modulation of Active Sites to Promote Electrocatalytic Oxygen Evolution. Advanced Materials. https://doi.org/10.1002/adma.202200270
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