The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Rechargeable Zinc–Air Batteries with an Ultralarge Discharge Capacity per Cycle and an Ultralong Cycle Life
Open accessAbstract
A conventional two‐electrode rechargeable zinc–air battery (RZAB) has two major problems: 1) opposing requirements for the oxygen reduction (ORR) and oxygen evolution (OER) reactions from the catalyst at the air cathode; and 2) zinc‐dendrite formation, hydrogen generation, and zinc corrosion at the zinc anode. To tackle these problems, a three‐electrode RZAB (T‐RZAB) including a hydrophobic discharge cathode, a hydrophilic charge cathode, and a zinc‐free anode is developed. The decoupled cathodes enable fast ORR and OER kinetics, and avoid oxidization of the ORR catalyst. The zinc‐free anode using tin‐coated copper foam that induces the growth of (002)Zn planes, suppresses hydrogen evolution, and prevents Zn corrosion. As a result, the T‐RZABs have a high discharge capacity per cycle of 800 mAh cm−2, a low voltage gap between the discharge/charge platforms of 0.66 V, and an ultralong cycle life of 5220 h at a current density of 10 mA cm−2. A large T‐RZAB with a discharge capacity of 10 Ah per cycle with no obvious degradation after cycling for 1000 h is developed. Finally, a T‐RZAB pack that has an energy density of 151.8 Wh kg−1 and a low cost of 46.7 US dollars kWh−1 is assembled.
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Cites
Liu, S., Li, C., Zachman, M. J., Zeng, Y., Yu, H., Li, B., Wang, M., Braaten, J., Liu, J., Meyer, H. M., et al. (2022) · Nature Energy · doi:10.1038/s41560-022-01062-1 · Cited by 733
Self-citationAnalysis of the limitations in the oxygen reduction activity of transition metal oxide surfaces
Li, H., Kelly, S., Guevarra, D., Wang, Z., Wang, Y., Haber, J. A., Anand, M., Gunasooriya, G. T. K. K., Abraham, C. S., Vijay, S., et al. (2021) · Nature Catalysis · doi:10.1038/s41929-021-00618-w · Cited by 341
Zhou, W., Su, H., Cheng, W., Li, Y., Jiang, J., Liu, M., Yu, F., Wang, W., Wei, S., & Liu, Q. (2022) · Nature Communications · doi:10.1038/s41467-022-34169-w · Cited by 264
Cited by
Zn-based batteries for sustainable energy storage: strategies and mechanisms
Tang, L., Peng, H., Kang, J., Chen, H., Zhang, M., Liu, Y., Kim, D. H., Liu, Y., & Lin, Z. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00295k · Cited by 548
A Review of Rechargeable Zinc–Air Batteries: Recent Progress and Future Perspectives
Nazir, G., Rehman, A., Lee, J.-H., Kim, C.-H., Gautam, J., Heo, K., Hussain, S., Ikram, M., AlObaid, A. A., Lee, S.-Y., et al. (2024) · Nano-Micro Letters · doi:10.1007/s40820-024-01328-1 · Cited by 328
Metadata
- Authors
- Zhong, X., Shao, Y., Chen, B., Li, C., Sheng, J., Xiao, X., Xu, B., Li, J., Cheng, H., & Zhou, G.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2023-06-06
- Volume
- 35
- Issue
- 30
- Pages
- e2301952-e2301952
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W4366083624
- Cited by
- 178
- References
- 3
- FWCI
- 13.05
- Type
- journal article
- Language
- en
- Open access
- bronze
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- The paper
- Zhong, X., Shao, Y., Chen, B., Li, C., Sheng, J., Xiao, X., Xu, B., Li, J., Cheng, H., & Zhou, G. (2023). Rechargeable Zinc–Air Batteries with an Ultralarge Discharge Capacity per Cycle and an Ultralong Cycle Life. Advanced Materials. https://doi.org/10.1002/adma.202301952
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