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Studies on Thermoelectric Properties of n‐type Polycrystalline SnSe1‐xSx by Iodine Doping
Open accessAbstract
Iodine‐doped n‐type SnSe polycrystalline by melting and hot pressing is prepared. The prepared material is anisotropic with a peak ZT of ≈0.8 at about 773 K measured along the hot pressing direction. This is the first report on thermoelectric properties of n‐type Sn chalcogenide alloys. With increasing content of iodine, the carrier concentration changed from 2.3 × 10 17 cm−3 (p‐type) to 5.0 × 10 15 cm−3 (n‐type) then to 2.0 × 10 17 cm−3 (n‐type). The decent ZT is mainly attributed to the intrinsically low thermal conductivity due to the high anharmonicity of the chemical bonds like those in p‐type SnSe. By alloying with 10 at% SnS, even lower thermal conductivity and an enhanced Seebeck coefficient were achieved, leading to an increased ZT of ≈1.0 at about 773 K measured also along the hot pressing direction.
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Cites
Topological crystalline insulators in the SnTe material class
Hsieh, T. H., Lin, H., Liu, J., Duan, W., Bansil, A., & Fu, L. (2012) · Nature Communications · doi:10.1038/ncomms1969 · Cited by 1,449
Resonant bonding leads to low lattice thermal conductivity
Lee, S., Esfarjani, K., Luo, T., Zhou, J., Tian, Z., & Chen, G. (2014) · Nature Communications · doi:10.1038/ncomms4525 · Cited by 679
Self-citation
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Ultrahigh power factor and thermoelectric performance in hole-doped single-crystal SnSe
Zhao, L.-D., Tan, G., Hao, S., He, J., Pei, Y., Chi, H., Wang, H., Gong, S., Xu, H., Dravid, V. P., et al. (2016) · Science · doi:10.1126/science.aad3749 · Cited by 2,037
Mao, J., Liu, Z., Zhou, J., Zhu, H., Zhang, Q., Chen, G., & Ren, Z. (2018) · Advances in Physics · doi:10.1080/00018732.2018.1551715 · Cited by 592
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Shi, X., Chen, L., & Uher, C. (2016) · International Materials Reviews · doi:10.1080/09506608.2016.1183075 · Cited by 494
Metadata
- Authors
- Zhang, Q., Chere, E. K., Sun, J., Cao, F., Dahal, K., Chen, S., Chen, G., & Ren, Z.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2015-04-22
- Volume
- 5
- Issue
- 12
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2107274567
- Cited by
- 321
- References
- 2
- FWCI
- 18.39
- Type
- journal article
- Language
- en
- Open access
- green
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- Zhang, Q., Chere, E. K., Sun, J., Cao, F., Dahal, K., Chen, S., Chen, G., & Ren, Z. (2015). Studies on Thermoelectric Properties of n‐type Polycrystalline SnSe1‐xSx by Iodine Doping. Advanced Energy Materials. https://doi.org/10.1002/aenm.201500360
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