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Facile Synthesis of Crumpled Nitrogen‐Doped MXene Nanosheets as a New Sulfur Host for Lithium–Sulfur Batteries
Open accessAbstract
Crumpled nitrogen‐doped MXene nanosheets with strong physical and chemical coadsorption of polysulfides are synthesized by a novel one‐step approach and then utilized as a new sulfur host for lithium–sulfur batteries. The nitrogen‐doping strategy enables introduction of heteroatoms into MXene nanosheets and simultaneously induces a well‐defined porous structure, high surface area, and large pore volume. The as‐prepared nitrogen‐doped MXene nanosheets have a strong capability of physical and chemical dual‐adsorption for polysulfides and achieve a high areal sulfur loading of 5.1 mg cm–2. Lithium–sulfur batteries, based on crumpled nitrogen‐doped MXene nanosheets/sulfur composites, demonstrate outstanding electrochemical performances, including a high reversible capacity (1144 mA h g–1 at 0.2C rate) and an extended cycling stability (610 mA h g–1 at 2C after 1000 cycles).
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Cited by
Recent Advances in Oxidation Stable Chemistry of 2D MXenes
Cao, F., Zhang, Y., Wang, H., Khan, K., Tareen, A. K., Qian, W., Zhang, H., & Ågren, H. (2022) · Advanced Materials · doi:10.1002/adma.202107554 · Cited by 648
Xiu, L., Wang, Z., Yu, M., Wu, X., & Qiu, J. (2018) · ACS Nano · doi:10.1021/acsnano.8b02849 · Cited by 588
Du, C., Dinh, K. N., Liang, Q., Zheng, Y., Luo, Y., Zhang, J., & Yan, Q. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201801127 · Cited by 274
Liu, H., Hu, Z., Liu, Q., Sun, P., Wang, Y., Chou, S., Hu, Z., & Zhang, Z. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta09538a · Cited by 176
Wang, Y., Sun, J., Qian, X., Zhang, Y., Yu, L., Niu, R., Zhao, H., & Zhu, J. (2019) · Journal of Power Sources · doi:10.1016/j.jpowsour.2019.01.036 · Cited by 136
Metadata
- Authors
- Bao, W., Liu, L., Wang, C., Choi, S., Wang, D., & Wang, G.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-01-11
- Volume
- 8
- Issue
- 13
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2784270919
- Cited by
- 745
- References
- 0
- FWCI
- 33.30
- Type
- journal article
- Language
- en
- Open access
- green
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- Bao, W., Liu, L., Wang, C., Choi, S., Wang, D., & Wang, G. (2018). Facile Synthesis of Crumpled Nitrogen‐Doped MXene Nanosheets as a New Sulfur Host for Lithium–Sulfur Batteries. Advanced Energy Materials. https://doi.org/10.1002/aenm.201702485
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