Cited by 377Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsFuel Cells and Related Materials

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Ultrafine Pt Nanoparticle‐Decorated Pyrite‐Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting

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Han, Xiaopeng, Wu, Xiaoyu, Deng, Yida, Liu, Jian, Lu, Jun, Zhong, Cheng, Hu, Wenbin·2018·Advanced Energy Materials

DOI 10.1002/aenm.201800935

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Abstract

Abstract To improve the utilization efficiency of precious metals, metal‐supported materials provide a direction for fabricating highly active and stable heterogeneous catalysts. Herein, carbon cloth (CC)‐supported Earth‐abundant CoS 2 nanosheet arrays (CoS 2 /CC) are presented as ideal substrates for ultrafine Pt deposition (Pt‐CoS 2 /CC) to achieve remarkable performance toward the hydrogen and oxygen evolution reactions (HER/OER) in alkaline solutions. Notably, the Pt‐CoS 2 /CC hybrid delivers an overpotential of 24 mV at 10 mA cm −2 and a mass activity of 3.89 A Pt mg −1 , which is 4.7 times higher than that of commercial Pt/C, at an overpotential of 130 mV for catalyzing the HER. An alkali‐electrolyzer using Pt‐CoS 2 /CC as a bifunctional electrode enables a water‐splitting current density of 10 mA cm −2 at a low voltage of 1.55 V and can sustain for more than 20 h, which is superior to that of the state‐of‐the‐art Pt/C+RuO 2 catalyst. Further experimental and theoretical simulation studies demonstrate that strong electronic interaction between Pt and CoS 2 synergistically optimize hydrogen adsorption/desorption behaviors and facilitate the in situ generation of OER active species, enhancing the overall water‐splitting performance. This work highlights the regulation of interfacial and electronic synergy in pursuit of highly efficient and durable supported catalysts for hydrogen and oxygen electrocatalytic applications.

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Authors: Han, X., Wu, X., Deng, Y., Liu, J., Lu, J., Zhong, C., & Hu, W.
Affiliations: Tianjin University (CN)
Shandong University (CN)
Argonne National Laboratory (US)
Corresponding author: Zhong, Cheng
Hu, Wenbin
ORCID: Han, Xiaopeng
Wu, Xiaoyu
Deng, Yida
Liu, Jian
Lu, Jun
Zhong, Cheng
Hu, Wenbin
Venue: Advanced Energy Materials
Publisher: Wiley
Published: 2018-07-02
Volume: 8
Issue: 24
ISSN: 1614-6832 (ISSN-L)
1614-6840
DOI: 10.1002/aenm.201800935
OpenAlex: W2810461784
Cited by: 375
References: 87
Citations by year: 2026: 19 · 2025: 23 · 2024: 28 · 2023: 32 · 2022: 49 · 2021: 75 · 2020: 73 · 2019: 69 · 2018: 7
FWCI: 12.94
Type: journal article
Language: en
Open access: green
www.osti.gov
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Advanced Energy Materials (publishedVersion)
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Funders: National Natural Science Foundation of China (51602216, 51771134, 51472178, 51571151)
Natural Science Foundation of Guangdong Province (U1601216)
Natural Science Foundation of Tianjin City (17JCQNJC02100, 16JCYBJC17600)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Keywords: carbon cloth support, bifunctional electrocatalysts, hydrogen evolution reaction, oxygen evolution reaction, overall water splitting, alkaline electrolyzer, hydrogen adsorption, earth-abundant catalysts

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Ultrafine Pt Nanoparticle‐Decorated Pyrite‐Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting

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