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A Room‐Temperature Molten Hydrate Electrolyte for Rechargeable Zinc–Air Batteries
Open accessAbstract
Aqueous Zn‐based batteries are attracting extensive interest because of their economic feasibility and potentially high energy density. However, poor rechargeability of Zn anode in conventional electrolytes resulting from dendrite formation and self‐corrosion hinders their practical implementation. Herein, a Zn molten hydrate composed of inorganic Zn salt and water is demonstrated as an advantageous electrolyte for solving these issues. In this electrolyte, dendrite‐free Zn deposition/dissolution reaction with a high Coulombic efficiency (≈99%) as well as long‐term stability, free from CO 2 poisoning are realized. The resultant Zn–air cell exhibits a reversible capacity of 1000 mAh g(catalyst)−1 over 100 cycles at 30 °C. Combined with the intrinsic safety associated with aqueous chemistry and cost benefit of the raw material, the present Zn–air battery makes a strong candidate for large‐scale energy storage.
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Citations
Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Cited by
A rechargeable zinc-air battery based on zinc peroxide chemistry
Sun, W., Wang, F., Zhang, B., Zhang, M., Küpers, V., Ji, X., Theile, C., Bieker, P., Xu, K., Wang, C., et al. (2021) · Science · doi:10.1126/science.abb9554 · Cited by 1,082
Recent Progress on Zn Anodes for Advanced Aqueous Zinc‐Ion Batteries
Nie, C., Wang, G., Wang, D., Wang, M., Gao, X., Bai, Z., Wang, N., Yang, J., Xing, Z., & Dou, S. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300606 · Cited by 561
Wang, C., Pei, Z., Meng, Q., Zhang, C., Sui, X., Yuan, Z., Wang, S., & Chen, Y. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202012030 · Cited by 394
Metadata
- Authors
- Chen, C., Matsumoto, K., Kubota, K., Hagiwara, R., & Xu, Q.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2019-04-16
- Volume
- 9
- Issue
- 22
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2939018111
- Cited by
- 217
- References
- 2
- FWCI
- 9.87
- Type
- journal article
- Language
- en
- Open access
- green
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- Chen, C., Matsumoto, K., Kubota, K., Hagiwara, R., & Xu, Q. (2019). A Room‐Temperature Molten Hydrate Electrolyte for Rechargeable Zinc–Air Batteries. Advanced Energy Materials. https://doi.org/10.1002/aenm.201900196
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