The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
A Novel Dendrite‐Free Mn2+/Zn2+ Hybrid Battery with 2.3 V Voltage Window and 11000‐Cycle Lifespan
Abstract
With the increasing energy crisis and environmental pollution, rechargeable aqueous Zn‐based batteries (AZBs) are receiving unprecedented attention due to their list of merits, such as low cost, high safety, and nontoxicity. However, the limited voltage window, Zn dendrites, and relatively low specific capacity are still great challenges. In this work, a new reaction mechanism of reversible Mn 2+ ion oxidation deposition is introduced to AZBs. The assembled Mn 2+/Zn 2+ hybrid battery (Mn 2+/Zn 2+ HB) based on a hybrid storage mechanism including Mn 2+ ion deposition, Zn 2+ ion insertion, and conversion reaction of MnO 2 can achieve an ultrawide voltage window (0–2.3 V) and high capacity (0.96 mAh cm−2). Furthermore, the carbon nanotubes coated Zn anode is proved to effectively inhibit Zn dendrites and control side reaction, hence exhibiting an ultrastable cycling (33 times longer than bare Zn foil) without obvious polarization. Benefiting from the optimal Zn anode and highly reversible Mn 2+/Zn 2+ hybrid storage mechanism, the Mn 2+/Zn 2+ HB shows an excellent cycling performance over 11 000 cycles with a 100% capacity retention. To the best of the authors' knowledge, it is the highest reported cycling performance and wide voltage window for AZBs with mild electrolyte, which may inspire a great insight into designing high‐performance aqueous batteries.
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Xu, L., & Salmeron, M. (1998) · Langmuir · doi:10.1021/la980529y · Cited by 74
Cited by
Li, M., Li, Z., Wang, X., Meng, J., Liu, X., Wu, B., Han, C., & Mai, L. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00030f · Cited by 559
Self-citationAdvances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
An Overview and Future Perspectives of Rechargeable Zinc Batteries
Shi, Y., Chen, Y., Shi, L., Wang, K., Wang, B., Li, L., Ma, Y., Li, Y., Sun, Z., Ali, W., et al. (2020) · Small · doi:10.1002/smll.202000730 · Cited by 389
Strategies towards the challenges of zinc metal anode in rechargeable aqueous zinc ion batteries
Wang, J., Yang, Y., Zhang, Y., Li, Y., Sun, R., Wang, Z., & Wang, H. (2021) · Energy Storage Materials · doi:10.1016/j.ensm.2020.10.027 · Cited by 359
Self-citationAnode for Zinc-Based Batteries: Challenges, Strategies, and Prospects
Lu, W., Zhang, C., Zhang, H., & Li, X. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.1c00939 · Cited by 355
Metadata
- Authors
- Li, M., He, Q., Li, Z., Li, Q., Zhang, Y., Meng, J., Liu, X., Li, S., Wu, B., Chen, L., Liu, Z., Luo, W., Han, C., & Mai, L.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2019-06-26
- Volume
- 9
- Issue
- 29
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2954360858
- Cited by
- 238
- References
- 1
- FWCI
- 12.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, M., He, Q., Li, Z., Li, Q., Zhang, Y., Meng, J., Liu, X., Li, S., Wu, B., Chen, L., Liu, Z., Luo, W., Han, C., & Mai, L. (2019). A Novel Dendrite‐Free Mn2+/Zn2+ Hybrid Battery with 2.3 V Voltage Window and 11000‐Cycle Lifespan. Advanced Energy Materials. https://doi.org/10.1002/aenm.201901469
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