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Visible‐Light‐Driven Hydrogen Evolution Using Planarized Conjugated Polymer Photocatalysts
Open accessAbstract
Linear poly(p‐phenylene)s are modestly active UV photocatalysts for hydrogen production in the presence of a sacrificial electron donor. Introduction of planarized fluorene, carbazole, dibenzo[b,d]thiophene or dibenzo[b,d]thiophene sulfone units greatly enhances the H 2 evolution rate. The most active dibenzo[b,d]thiophene sulfone co‐polymer has a UV photocatalytic activity that rivals TiO 2, but is much more active under visible light. The dibenzo[b,d]thiophene sulfone co‐polymer has an apparent quantum yield of 2.3 % at 420 nm, as compared to 0.1 % for platinized commercial pristine carbon nitride.
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Cites
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Cited by
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
Wan, Y., Wang, L., Xu, H., Wu, X., & Yang, J. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00564 · Cited by 363
Metadata
- Authors
- Sprick, R. S., Bonillo, B., Clowes, R., Guiglion, P., Brownbill, N. J., Slater, B. J., Blanc, F., Zwijnenburg, M. A., Adams, D. J., & Cooper, A. I.
- Venue
- Angewandte Chemie
- Publisher
- Wiley
- Published
- 2015-12-22
- Volume
- 128
- Issue
- 5
- Pages
- 1824-1828
- ISSN
- 0044-8249 (ISSN-L)
- 1521-3757
- OpenAlex
- W4210394271
- Cited by
- 177
- References
- 1
- FWCI
- 5.57
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Sprick, R. S., Bonillo, B., Clowes, R., Guiglion, P., Brownbill, N. J., Slater, B. J., Blanc, F., Zwijnenburg, M. A., Adams, D. J., & Cooper, A. I. (2016). Visible‐Light‐Driven Hydrogen Evolution Using Planarized Conjugated Polymer Photocatalysts. Angewandte Chemie. https://doi.org/10.1002/ange.201510542
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