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Selective Isomerization of Hydrocarbon Chains on External Surfaces of Zeolite Crystals
Abstract
A mechanism has been found that explains the distribution of products obtained in the isomerizations of long-chain alkanes on ZSM-22 and SAPO-11 catalysts so well that it should now be possible to tailor reactions for the synthesis of branched hydrocarbons. The reactions occur at the external surface of the catalyst according to a lock-and-key model (shown on the right); thus, the classical concept of shape-selective catalysis within micropores is substantially extended.
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Cited by
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Shamzhy, M., Opanasenko, M., Concepción, P., & Martínez, A. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00887f · Cited by 508
Toward the Atomic Scale Simulation of Intricate Acidic Aluminosilicate Catalysts
Chizallet, C. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01136 · Cited by 79
Treps, L., Gomez, A., de Bruin, T., & Chizallet, C. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05103 · Cited by 63
Spectroscopic Expression of the External Surface Sites of H-ZSM-5
Treps, L., Demaret, C., Wisser, D., Harbuzaru, B., Méthivier, A., Guillon, E., Benedis, D. V., Gomez, A., Bruin, T. D., Rivallan, M., et al. (2021) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.0c10200 · Cited by 63
Ab Initio Simulation of the Acid Sites at the External Surface of Zeolite Beta
Rey, J., Raybaud, P., & Chizallet, C. (2017) · ChemCatChem · doi:10.1002/cctc.201700080 · Cited by 49
Metadata
- Authors
- Martens, J. A., Souverijns, W., Verrelst, W., Parton, R., Froment, G. F., & Jacobs, P. A.
- Venue
- Angewandte Chemie International Edition in English
- Publisher
- Wiley
- Published
- 1995-12
- Volume
- 34
- Issue
- 22
- Pages
- 2528-2530
- ISSN
- 0570-0833 (ISSN-L)
- OpenAlex
- W2154784480
- Cited by
- 213
- References
- 0
- FWCI
- 6.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Selective Isomerization of Hydrocarbon Chains on External Surfaces of Zeolite Crystals. https://app.cochat.ai/papers/10.1002/anie.199525281
- The paper
- Martens, J. A., Souverijns, W., Verrelst, W., Parton, R., Froment, G. F., & Jacobs, P. A. (1995). Selective Isomerization of Hydrocarbon Chains on External Surfaces of Zeolite Crystals. Angewandte Chemie International Edition in English. https://doi.org/10.1002/anie.199525281
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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