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Water Oxidation Catalyzed by a Dinuclear Mn Complex: A Functional Model for the Oxygen‐Evolving Center of Photosystem II
Open accessAbstract
A highly specific and catalytic oxidation of water occurs when using a dinuclear Mn complex of a mononegative carboxylate-containing pentadentate ligand (see scheme). Isotope-labeling experiments coupled with membrane inlet mass spectrometry show that one oxygen atom in the evolved O2 molecule is derived from water and the other from the oxidant.
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Citations
Cited by
Proton-coupled electron transfer
Huynh, M. H. V., & Meyer, T. J. (2007) · Chemical Reviews · doi:10.1021/cr0500030 · Cited by 1,659
Artificial Photosynthesis: Molecular Systems for Catalytic Water Oxidation
Kärkäs, M. D., Verho, O., Johnston, E. V., & Åkermark, B. (2014) · Chemical Reviews · doi:10.1021/cr400572f · Cited by 1,376
Molecular Catalysts for Water Oxidation
Blakemore, J. D., Crabtree, R. H., & Brudvig, G. W. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00122 · Cited by 1,150
Development of Bioinspired Mn4O4−Cubane Water Oxidation Catalysts: Lessons from Photosynthesis
Dismukes, G. C., Brimblecombe, R., Felton, G. A. N., Pryadun, R. S., Sheats, J. E., Spiccia, L., & Swiegers, G. F. (2009) · Accounts of Chemical Research · doi:10.1021/ar900249x · Cited by 549
Energy Conversion in Natural and Artificial Photosynthesis
McConnell, I., Li, G., & Brudvig, G. W. (2010) · Chemistry & Biology · doi:10.1016/j.chembiol.2010.05.005 · Cited by 440
Metadata
- Authors
- Poulsen, A. K., Rompel, A., & McKenzie, C. J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2005-10-25
- Volume
- 44
- Issue
- 42
- Pages
- 6916-6920
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2100429960
- Cited by
- 214
- References
- 0
- FWCI
- 7.88
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Poulsen, A. K., Rompel, A., & McKenzie, C. J. (2005). Water Oxidation Catalyzed by a Dinuclear Mn Complex: A Functional Model for the Oxygen‐Evolving Center of Photosystem II. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200502114
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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