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Chemical Synthesis of Mesoporous Carbon Nitrides Using Hard Templates and Their Use as a Metal‐Free Catalyst for Friedel–Crafts Reaction of Benzene
Abstract
In the footsteps of Liebig and Berzelius: A material first synthesized in 1834, carbon nitride (C3N4), was synthesized in a graphitic mesoporous form by using silica nanoparticles as templates. The resulting electron-rich solid is an active catalyst for the Friedel–Crafts acylation of benzene with hexanoyl chloride. Presumably the catalysis arises from a shift of electron density from the MOs of the catalyst to the unoccupied orbitals of benzene (see picture).
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Cites
Density-functional thermochemistry. III. The role of exact exchange
Becke, A. D. (1993) · The Journal of Chemical Physics · doi:10.1063/1.464913 · Cited by 103,767
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Thomas, A., Fischer, A., Goettmann, F., Antonietti, M., Müller, J.-O., Schlögl, R., & Carlsson, J. M. (2008) · Journal of Materials Chemistry · doi:10.1039/b800274f · Cited by 3,419
Self-citationDong, G., Zhang, Y., Pan, Q., & Qiu, J. (2014) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2014.04.002 · Cited by 1,085
Wei, J., Zhou, D., Sun, Z., Deng, Y., Xia, Y., & Zhao, D. (2013) · Advanced Functional Materials · doi:10.1002/adfm.201202764 · Cited by 931
Two‐Dimensional Polymers: Just a Dream of Synthetic Chemists?
Sakamoto, J., van Heijst, J., Lukin, O., & Schlüter, A. D. (2009) · Angewandte Chemie International Edition · doi:10.1002/anie.200801863 · Cited by 734
Metadata
- Authors
- Goettmann, F., Fischer, A., Antonietti, M., & Thomas, A.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2006-06-28
- Volume
- 45
- Issue
- 27
- Pages
- 4467-4471
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W1966805111
- Cited by
- 1,002
- References
- 1
- FWCI
- 12.80
- Type
- journal article
- Language
- en
- Open access
- closed
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- Goettmann, F., Fischer, A., Antonietti, M., & Thomas, A. (2006). Chemical Synthesis of Mesoporous Carbon Nitrides Using Hard Templates and Their Use as a Metal‐Free Catalyst for Friedel–Crafts Reaction of Benzene. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200600412
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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