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First‐Principles Considerations in the Design of Pd‐Alloy Catalysts for Oxygen Reduction
Abstract
The enhanced catalytic activity of Pd-alloy catalysts in oxygen reduction and the “volcano” relationship between activity and degree of alloying were studied by experiment and DFT calculations. Catalytic activity correlates with adsorption energy (AE) of Oads, which in turn depends on lattice strain (a/a0) due to alloying. A guideline for the rational design of such catalysts (see picture) predicts that a Pd11Fe alloy will have similar activity to Pt.
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Cited by
Recent Advances in Electrocatalysts for Oxygen Reduction Reaction
Shao, M., Chang, Q., Dodelet, J.-P., & Chenitz, R. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00462 · Cited by 3,903
Recent advancements in Pt and Pt-free catalysts for oxygen reduction reaction
Nie, Y., Li, L., & Wei, Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00484a · Cited by 2,156
Recent advances in catalysts for direct methanol fuel cells
Zhao, X., Yin, M., Ma, L., Liang, L., Liu, C., Liao, J., Lu, T., & Xing, W. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01307f · Cited by 939
Wang, J. X., Inada, H., Wu, L., Zhu, Y., Choi, Y., Liu, P., Zhou, W.-P., & Adzic, R. R. (2009) · Journal of the American Chemical Society · doi:10.1021/ja9067645 · Cited by 719
Bezerra, C. W. B., Zhang, L., Liu, H., Lee, K., Marques, A. L. B., Marques, E. P., Wang, H., & Zhang, J. (2007) · Journal of Power Sources · doi:10.1016/j.jpowsour.2007.08.028 · Cited by 439
Metadata
- Authors
- Suo, Y., Zhuang, L., & Lu, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2007-04-05
- Volume
- 46
- Issue
- 16
- Pages
- 2862-2864
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2097706822
- Cited by
- 276
- References
- 0
- FWCI
- 10.79
- Type
- journal article
- Language
- en
- Open access
- closed
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