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An All‐Inorganic, Stable, and Highly Active Tetraruthenium Homogeneous Catalyst for Water Oxidation
Abstract
Oxidation without organics: A tetraruthenium polyoxometalate (see picture; Ru blue, O red, Si yellow, W black) catalyzes the rapid oxidation of H2O to O2 in water at ambient temperature, and shows considerable stability under turnover conditions. The complex was characterized by several methods, including X-ray crystallography and cyclic voltammetry.
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
Density functional theory for transition metals and transition metal chemistry
Cramer, C. J., & Truhlar, D. G. (2009) · Physical Chemistry Chemical Physics · doi:10.1039/b907148b · Cited by 1,648
Efficient water oxidation at carbon nanotube–polyoxometalate electrocatalytic interfaces
Toma, F. M., Sartorel, A., Iurlo, M., Carraro, M., Parisse, P., Maccato, C., Rapino, S., Gonzalez, B. R., Amenitsch, H., Da Ros, T., et al. (2010) · Nature Chemistry · doi:10.1038/nchem.761 · Cited by 503
Cai, Q., Gao, R., Wang, Y., Xing, J., Zhang, Q., Zhu, M., Qin, X., Liao, M., & Huang, Y. (2025) · Polyoxometalates · doi:10.26599/pom.2024.9140083 · Cited by 22
Metadata
- Authors
- Geletii, Y. V., Botar, B., Kögerler, P., Hillesheim, D. A., Musaev, D. G., & Hill, C. L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2008-05-06
- Volume
- 47
- Issue
- 21
- Pages
- 3896-3899
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2140917975
- Cited by
- 592
- References
- 0
- FWCI
- 34.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Geletii, Y. V., Botar, B., Kögerler, P., Hillesheim, D. A., Musaev, D. G., & Hill, C. L. (2008). An All‐Inorganic, Stable, and Highly Active Tetraruthenium Homogeneous Catalyst for Water Oxidation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200705652
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